Publications related to Fission product yield

Atomic level insight into irradiation effects in nuclear fuel materials

Microstructural evolution during in-pile irradiation, radiation damage effects and fission products behavior in UO2 nuclear fuel are key issues in understanding and for the modeling of the performance as well as safety characteristics of nuclear fuels in t ...

EPFL2024

Gamma-ray Spectroscopy in Low-Power Nuclear Research Reactors

Andreas Pautz, Vincent Pierre Lamirand, Oskari Ville Pakari

Gamma-ray spectroscopy is an effective technique for radioactive material characterization, routine inventory verification, nuclear safeguards, health physics, and source search scenarios. Gamma-ray spectrometers typically cannot be operated in the immedia ...

MDPI2024

Probing Water Dissociation and Oxygen Replacement on Partially Oxygen-Covered Cu(111) by Reflection Absorption Infrared Spectroscopy

Rainer Beck, Mateusz Suchodol, Harmina Vejayan

The presence of chemisorbed oxygen on the Cu(111) surface is known to strongly reduce the activation barrier for water dissociation as compared to bare Cu(111). Here, we present direct experimental evidence for the hydrogen abstraction mechanism responsibl ...

2023

Cycloalkane Oxidation Catalyzed by Copper-based Catalysts with H2O2 under Mild Conditions

Nukorn Plainpan, Jantira Chimlert

Copper-catalyzed cycloalkane oxidation using H2O2 as an oxidant was investigated under mild conditions. The copper catalysts studied in this work ranged from commercially-available copper(II) salts to copper(II) complexes containing polypyridyl ligands. Va ...

WILEY-V C H VERLAG GMBH2023

Direct conversion of lignin to functionalized diaryl ethers via oxidative cross-coupling

Paul Joseph Dyson, Mingyang Liu

Efficient valorization of lignin, a sustainable source of functionalized aromatic products, would reduce dependence on fossil-derived feedstocks. Oxidative depolymerization is frequently applied to lignin to generate phenolic mono- mers. However, due to th ...

Nature Research2023

Search for Higgs boson and observation of Z boson through their decay into a charm quark-antiquark pair in boosted topologies in proton-proton collisions at √s=13 TeV

Matthias Finger, Konstantin Androsov, Qian Wang, Jan Steggemann, Anna Mascellani, Yiming Li, Varun Sharma, Xin Chen, Rakesh Chawla, Matteo Galli, Jian Wang, João Miguel das Neves Duarte, Tagir Aushev, Matthias Wolf, Yi Zhang, Lei Zhang, Tian Cheng, Yixing Chen, Werner Lustermann, Andromachi Tsirou, Alexis Kalogeropoulos, Andrea Rizzi, Ioannis Papadopoulos, Paolo Ronchese, Hua Zhang, Leonardo Cristella, Siyuan Wang, Tao Huang, David Vannerom, Michele Bianco, Sebastiana Gianì, Sun Hee Kim, Davide Di Croce, Kun Shi, Wei Shi, Abhisek Datta, Jian Zhao, Federica Legger, Gabriele Grosso, Ji Hyun Kim, Donghyun Kim, , , , , , , , , , , , , , , , , , , , , , , , , , , , , ,

Microlens-enhanced silicon photomultiplier arrays for LHCb SciFi Tracker Upgrade Ib

Olivier Schneider, Guido Haefeli, Ettore Zaffaroni, Carina Trippl

A large-scale Scintillating Fibre Tracker has been developed and constructed for the current LHCb Upgrade 1. The high radiation by fast neutrons reduces the light yield of the detector in the course of LHC Run 3, and is challenging the tracker's hit detect ...

ELSEVIER2022

Interface Tracking Investigation of the Sliding Bubbles Effects on Heat Transfer in the Laminar Regime

Konstantin Mikityuk, Lubomír Bures

Helium gases are utilized to remove fission products from the molten salt fast reactor (MSFR) core during operation. Helium gases and other volatile fission products may be introduced into the intermediate heat exchanger channels. The effect of these gases ...

2022

Towards the Validation of Noise Experiments in the CROCUS Reactor Using the TRIPOLI-4 Monte Carlo Code in Analog Mode

Andreas Pautz, Vincent Pierre Lamirand, Oskari Ville Pakari

Intrinsic neutron noise experiments offer a non-invasive manner to measure the prompt decay constant or reactivity of fissile systems. Using the fluctuations in the density of fission chains, one can infer the kinetics parameters via correlation analysis s ...

2021

Guidelines for performing lignin-first biorefining

Jeremy Luterbacher, Feng Wang

The valorisation of the plant biopolymer lignin is now recognised as essential to enabling the economic viability of the lignocellulosic biorefining industry. In this context, the "lignin-first" biorefining approach, in which lignin valorisation is conside ...

2021

Experimental validation of an integrated modelling approach to neutron emission studies at JET

Henri Weisen

An integrated modelling methodology for the calculation of realistic plasma neutron sources for the JET tokamak has been developed. The computational chain comprises TRANSP plasma transport and DRESS neutron spectrum calculations, and their coupling to the ...

IOP Publishing Ltd2021

Data assimilation of post-irradiation examination data for fission yields from GEF

Andreas Pautz, Daniel Jerôme Siefman, Mathieu Hursin, Dimitri Rochman

Nuclear data, especially fission yields, create uncertainties in the predicted concentrations of fission products in spent fuel which can exceed engineering target accuracies. Herein, we present a new framework that extends data assimilation methods to bur ...

EDP SCIENCES S A2020

Data assimilation of post irradiation examination experiments to adjust fission yields

Andreas Pautz, Daniel Jerôme Siefman, Mathieu Hursin

Nuclear data, especially fission yields, create uncertainties in the predicted concentrations of fission products in spent fuel. Herein, we present a new framework that extends data assimilation methods to burnup simulations by using data from post-irradia ...

E D P SCIENCES2020

Nuclear data uncertainties for Swiss BWR spent nuclear fuel characteristics

Mathieu Hursin, Hakim Ferroukhi, Dimitri Rochman, Abdelhamid Dokhane, Alexander Vasiliev

The effect of nuclear data (fission yields, cross sections and emitted spectra) is quantified for spent nuclear fuel assemblies from a realistic boiling water reactor operated over 25 cycles. Nominal calculations are performed with the CASMO5, SIMULATE-3 a ...

2020

Synergistic ICRH and NBI Heating for Fast Ion Generation and Maximising Fusion Rate in Mixed Plasmas at JET

Henri Weisen

The studies of recent JET experiments in H/D approximate to 0.85/0.15 plasma (2.9T/2MA) in which neutron rate was enhanced by applying 2.5MW of ICRH using D-(D-NBI)-H three-ion scheme are reported. An extensive analysis of this novel heating scenario has b ...

AMER INST PHYSICS2020

The shear strength of Opalinus Clay shale in the remoulded state

Alessio Ferrari

The Opalinus Clay shale formation is considered as a potential host geomaterial for the Swiss deep geological repository for radioactive waste. It presents different facies and it is characterised by a multi-scale heterogeneous composition, by a typical fi ...

2020

Experimental and numerical study of stochastic branching noise in nuclear reactors

Oskari Ville Pakari

Noise analysis applied to nuclear reactor physics is a powerful tool to investigate a reactor's kinetic parameters, and more generally underlying physical processes determining core behavior. The kinetic parameters are the coefficients of simplified time-d ...

EPFL2020

Analysis of the sorption-enhanced chemical looping biomass gasification process: Performance assessment and optimization through design of experiment approach

François Maréchal, Thanaphorn Detchusananard

In this study, the performance of high-purity hydrogen production through the sorption-enhanced chemical looping gasification (SECLG) process, involving a gasifier, calciner, and air reactor, was investigated. In this process, the biomass feedstock was woo ...

2020

Determination of the activity inventory and associated uncertainty quantification for the CROCUS zero power research reactor

Andreas Pautz, Vincent Pierre Lamirand, Mathieu Hursin, DongHyuk Lee, Pavel Frajtag

The paper describes the source term estimation of CROCUS, the zero power research reactor of EPFL, to be used for dispersion analysis under accidental conditions. To fulfil regulatory requirements, the source term of the CROCUS fuel is estimated through Mo ...

2019

Development and Application of Data Assimilation Methods in Reactor Physics

Daniel Jerôme Siefman

Simulations of nuclear reactor physics can disagree significantly from experimental evidence, even when the most accurate models are used. An important part of this bias from experiment is caused by nuclear data. The nuclear data have inherent uncertaintie ...

EPFL2019