Publications related to Chemical transport model

Modular Multiplatform Compatible Air Measurement System (MoMuCAMS): a new modular platform for boundary layer aerosol and trace gas vertical measurements in extreme environments

Julia Schmale, Andrea Baccarini, Roman Pohorsky

The Modular Multiplatform Compatible Air Measurement System (MoMuCAMS) is a newly developed in situ aerosol and trace gas measurement platform for lower-atmospheric vertical profiling. MoMuCAMS has been primarily designed to be attached to a Helikite, a ru ...

2024

Low ozone dry deposition rates to sea ice during the MOSAiC field campaign: Implications for the Arctic boundary layer ozone budget

Julia Schmale, Ivo Fabio Beck, Hélène Paule Angot

Dry deposition to the surface is one of the main removal pathways of tropospheric ozone (O3). We quantified for the first time the impact of O3 deposition to the Arctic sea ice on the planetary boundary layer (PBL) O3 concentration and budget using year-ro ...

2023

Nitrogen oxides in the free troposphere: implications for tropospheric oxidants and the interpretation of satellite NO2 measurements

Ilann Ernest Valentin Bourgeois

Satellite-based retrievals of tropospheric NO(2)columns are widely used to infer NOx (equivalent to NO + NO2) emissions. These retrievals rely on model information for the vertical distribution of NO2. The free tropospheric background above 2 km is particu ...

Copernicus GmbH2023

Effects of simulated secondary organic aerosol water on PM 1 levels and composition over the US

Athanasios Nenes, Spyros Pandis

Water is a key component of atmospheric aerosol, affecting many aerosol processes including gas-to-particle partitioning of semi-volatile compounds. Water related to secondary organic aerosol (SOAW) is often neglected in atmospheric chemical transport mode ...

Copernicus GmbH2023

Aerosol and dynamical contributions to cloud droplet formation in Arctic low-level clouds

Athanasios Nenes, Ghislain Gilles Jean-Michel Motos, Paraskevi Georgakaki, Jörg Wieder, Guangyu Li

The Arctic is one of the most rapidly warming regions of the globe. Low-level clouds and fog modify the energy transfer from and to space and play a key role in the observed strong Arctic surface warming, a phenomenon commonly termed "Arctic amplification" ...

Copernicus GmbH2023

Improved extended-range prediction of persistent stratospheric perturbations using machine learning

Guillaume Romain Obozinski, Raphaël Gérard Théodore Michel Marie de Deloÿe et Fourcade de Fondeville

On average every 2 years, the stratospheric polar vortex exhibits extreme perturbations known as sudden stratospheric warmings (SSWs). The impact of these events is not limited to the stratosphere: but they can also influence the weather at the surface of ...

Copernicus Gesellschaft Mbh2023

A full year of aerosol size distribution data from the central Arctic under an extreme positive Arctic Oscillation: insights from the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition

Julia Schmale, Benjamin Jérémy Laurent Heutte, Jakob Boyd Pernov, Ivo Fabio Beck, Hélène Paule Angot, Lubna Dada, Federico Bianchi

The Arctic environment is rapidly changing due to accelerated warming in the region. The warming trend is driving a decline in sea ice extent, which thereby enhances feedback loops in the surface energy budget in the Arctic. Arctic aerosols play an importa ...

Copernicus Publications2023

Multiphase processes in the EC-Earth model and their relevance to the atmospheric oxalate, sulfate, and iron cycles

Athanasios Nenes

Understanding how multiphase processes affect the iron-containing aerosol cycle is key to predicting ocean biogeochemistry changes and hence the feedback effects on climate. For this work, the EC-Earth Earth system model in its climate-chemistry configurat ...

COPERNICUS GESELLSCHAFT MBH2022

A Downscaling Intercomparison Study: The Representation of Slope- and Ridge-Scale Processes in Models of Different Complexity

Varun Sharma, Franziska Gerber, Albertus Christiaan Kruyt, Dylan Stewart Reynolds

Spatially distributed meteorological information at the slope scale is relevant for many processes in complex terrain, yet information at this sub-km spatial resolution is difficult to obtain. While downscaling to kilometer resolutions is well described in ...

FRONTIERS MEDIA SA2022

Secondary aerosol formation during the dark oxidation of residential biomass burning emissions

Athanasios Nenes, Spyros Pandis

Particulate matter from biomass burning emissions affects air quality, ecosystems and climate; however, quantifying these effects requires that the connection between primary emissions and secondary aerosol production is firmly established. We performed at ...

ROYAL SOC CHEMISTRY2022

Introducing CRYOWRF v1.0: multiscale atmospheric flow simulations with advanced snow cover modelling

Varun Sharma, Michael Lehning, Franziska Gerber

Accurately simulating snow-cover dynamics and the snow-atmosphere coupling is of major importance for topics as wide-ranging as water resources, natural hazards and climate change impacts with consequences for sea-level rise. We present a new modelling fra ...

2023

System and method for privacy-preserving distributed training of machine learning models on distributed datasets

Jean-Pierre Hubaux, Juan Ramón Troncoso-Pastoriza, David Jules Froelicher, Apostolos Pyrgelis, Joao André Gomes de Sá e Sousa, Jean-Philippe Léonard Bossuat, Sinem Sav

A computer-implemented method and a distributed computer system (100) for privacy- preserving distributed training of a global model on distributed datasets (DS1 to DSn). The system has a plurality of data providers (DP1 to DPn) being communicatively coupl ...

2021

Acidity and the multiphase chemistry of atmospheric aqueous particles and clouds

Athanasios Nenes

The acidity of aqueous atmospheric solutions is a key parameter driving both the partitioning of semi-volatile acidic and basic trace gases and their aqueous-phase chemistry. In addition, the acidity of atmospheric aqueous phases, e.g., deliquesced aerosol ...

Copernicus GmbH2021

A multiphase CMAQ version 5.0 adjoint

Athanasios Nenes

We present the development of a multiphase adjoint for the Community Multiscale Air Quality (CMAQ) model, a widely used chemical transport model. The adjoint model provides location- and time-specific gradients that can be used in various applications such ...

2020

Direct numerical simulation of phase change in the presence of non-condensable gases

Lubomír Bures, Yohei Sato

This paper describes a new numerical method for the simulation of phase change phenomena between a liquid and a vapour in the presence of non-condensable gases. The method is based on an interface-tracking approach in the framework of single-fluid modellin ...

2020

Tracking Lagrangian transport in Lake Geneva: A 3D numerical modeling investigation

David Andrew Barry, Ulrich Lemmin, Andrea Cimatoribus

Lake Geneva, the largest freshwater lake in Western Europe, is subject to important environmental pressures from its densely populated shores and watershed. To maintain and improve water quality in this lake, as well as in other enclosed or semi‐enclosed b ...

American Society of Limnology and Oceanography2019

Effects of Atmospheric Processing on the Oxidative Potential of Biomass Burning Organic Aerosols

Athanasios Nenes, Kalliopi Violaki

Oxidative potential (OP), which is the ability of certain components in atmospheric particles to generate reactive oxidative species (ROS) and deplete antioxidants in vivo, is a prevailing toxicological mechanism underlying the adverse health effects assoc ...

AMER CHEMICAL SOC2019

Importance of the advection scheme for the simulation of water isotopes over Antarctica by atmospheric general circulation models: A case study for present-day and Last Glacial Maximum with LMDZ-iso

Etienne Gabriel Henri Vignon

Atmospheric general circulation models (AGCMs) are known to have a warm and isotopically enriched bias over Antarctica. We test here the hypothesis that these biases are partly consequences of a too diffusive advection. Exploiting the LMDZ-iso model, we sh ...

2019

Multi-scale modeling of the urban meteorology: Integration of a new canopy model in the WRF model

Dasaraden Mauree, Alain Clappier

Urban parametrizations have been recently developed and integrated in mesoscale meteorological models for a better reproduction of urban heat islands and to compute building energy consumption. The objective of the present study is to evaluate the value of ...

2018

Modeling the effects of future urban planning scenarios on the Urban Heat Island in a complex region

Jean-Louis Scartezzini, Dasaraden Mauree, Sylvain Labedens

Because of the global warming, urban planning strategies must be investigated to reduce the building energy consumption and increase the thermal comfort in cities. In the framework of Energy Strategy 2050 of Switzerland, this research aim to highlight the ...

2018