Publications related to Fission products (by element)

Atomic level insight into irradiation effects in nuclear fuel materials

Microstructural evolution during in-pile irradiation, radiation damage effects and fission products behavior in UO2 nuclear fuel are key issues in understanding and for the modeling of the performance as well as safety characteristics of nuclear fuels in t ...

EPFL2024

Gamma-ray Spectroscopy in Low-Power Nuclear Research Reactors

Andreas Pautz, Vincent Pierre Lamirand, Oskari Ville Pakari

Gamma-ray spectroscopy is an effective technique for radioactive material characterization, routine inventory verification, nuclear safeguards, health physics, and source search scenarios. Gamma-ray spectrometers typically cannot be operated in the immedia ...

MDPI2024

A concept for the extraction of the most refractory elements at CERN-ISOLDE as carbonyl complex ions

João Pedro Fernandes Pinto Ramos

We introduce a novel thick-target concept tailored to the extraction of refractory 4d and 5d transition metal radionuclides of molybdenum, technetium, ruthenium and tungsten for radioactive ion beam production. Despite the more than 60-year old history of ...

2022

Interface Tracking Investigation of the Sliding Bubbles Effects on Heat Transfer in the Laminar Regime

Konstantin Mikityuk, Lubomír Bures

Helium gases are utilized to remove fission products from the molten salt fast reactor (MSFR) core during operation. Helium gases and other volatile fission products may be introduced into the intermediate heat exchanger channels. The effect of these gases ...

2022

Towards the Validation of Noise Experiments in the CROCUS Reactor Using the TRIPOLI-4 Monte Carlo Code in Analog Mode

Andreas Pautz, Vincent Pierre Lamirand, Oskari Ville Pakari

Intrinsic neutron noise experiments offer a non-invasive manner to measure the prompt decay constant or reactivity of fissile systems. Using the fluctuations in the density of fission chains, one can infer the kinetics parameters via correlation analysis s ...

2021

High-Efficiency Deep-Red Light-Emitting Electrochemical Cell Based on a Trinuclear Ruthenium(II)-Silver(I) Complex

Mohammad Khaja Nazeeruddin

Turn-on time is a key factor for lighting devices to be of practical application. To decrease the turn-on time value of a deep-red light-emitting electrochemical cells (DR-LECs), two novel approaches based on molecularly engineered ruthenium phenanthroimid ...

AMER CHEMICAL SOC2021

Data assimilation of post-irradiation examination data for fission yields from GEF

Andreas Pautz, Daniel Jerôme Siefman, Mathieu Hursin, Dimitri Rochman

Nuclear data, especially fission yields, create uncertainties in the predicted concentrations of fission products in spent fuel which can exceed engineering target accuracies. Herein, we present a new framework that extends data assimilation methods to bur ...

EDP SCIENCES S A2020

Data assimilation of post irradiation examination experiments to adjust fission yields

Andreas Pautz, Daniel Jerôme Siefman, Mathieu Hursin

Nuclear data, especially fission yields, create uncertainties in the predicted concentrations of fission products in spent fuel. Herein, we present a new framework that extends data assimilation methods to burnup simulations by using data from post-irradia ...

E D P SCIENCES2020

Artificial Neural Networks as Surrogate Models for Uncertainty Quantification and Data Assimilation in 2-D/3-D Fuel Performance Studies

Andreas Pautz, Mathieu Hursin, Carlo Fiorina, Alessandro Scolaro, Daniel Jerôme Siefman

This paper preliminarily investigates the use of data-driven surrogates for fuel performance codes. The objective is to develop fast-running models that can be used in the frame of uncertainty quantification and data assimilation studies. In particular, da ...

2020

Nuclear data uncertainties for Swiss BWR spent nuclear fuel characteristics

Mathieu Hursin, Hakim Ferroukhi, Dimitri Rochman, Abdelhamid Dokhane, Alexander Vasiliev

The effect of nuclear data (fission yields, cross sections and emitted spectra) is quantified for spent nuclear fuel assemblies from a realistic boiling water reactor operated over 25 cycles. Nominal calculations are performed with the CASMO5, SIMULATE-3 a ...

2020

Efficient Kr/Xe separation from triangular g-C(3)N(4)nanopores, a simulation study

Nicola Marzari, Kumar Varoon Agrawal, Nicola Colonna, Davide Campi, Luis Francisco Villalobos Vazquez de la Parra

Poly(triazine imide) or PTI is a promising material for molecular sieving membranes, thanks to its atom-thick ordered lattice with an extremely high density (1.6 x 10(14)pores per cm(2)) of triangular-shaped nanopores of similar to 0.34 nm diameter. Here, ...

Royal Society of Chemistry2020

Determination of the activity inventory and associated uncertainty quantification for the CROCUS zero power research reactor

Andreas Pautz, Vincent Pierre Lamirand, Mathieu Hursin, DongHyuk Lee, Pavel Frajtag

The paper describes the source term estimation of CROCUS, the zero power research reactor of EPFL, to be used for dispersion analysis under accidental conditions. To fulfil regulatory requirements, the source term of the CROCUS fuel is estimated through Mo ...

2019

Development and Application of Data Assimilation Methods in Reactor Physics

Daniel Jerôme Siefman

Simulations of nuclear reactor physics can disagree significantly from experimental evidence, even when the most accurate models are used. An important part of this bias from experiment is caused by nuclear data. The nuclear data have inherent uncertaintie ...

EPFL2019

High-Fidelity Determination of Nuclide Inventories for Radioactive Waste Disposal

Valentyn Bykov

The general license application (RBG) for the Swiss deep geological repository will be submitted in 2024. Furthermore, the decommissioning of the nuclear power plants (NPPs) is coming soon, with the Mühleberg NPP (KKM) scheduled to shut down in 2019. In su ...

EPFL2019

Unraveling Thermodynamics, Stability, and Oxygen Evolution Activity of Strontium Ruthenium Perovskite Oxide

Nicola Marzari, Ivano Eligio Castelli, Xi Cheng

Extensive investigations in understanding the functional mechanisms of metal oxides behind oxygen evolution have been carried out since an electrolyzer has demonstrated promising possibilities as a device to produce hydrogen for electrochemical energy conv ...

Amer Chemical Soc2017

Mfn2 is critical for brown adipose tissue thermogenic function

Carlos Canto Alvarez, Joanna Ratajczak, Miriam Valera Alberni

Mitochondrial fusion and fission events, collectively known as mitochondrial dynamics, act as quality control mechanisms to ensure mitochondrial function and fine-tune cellular bioenergetics. Defective mitofusin 2 (Mfn2) expression and enhanced mitochondri ...

Wiley2017

Biogenic non-crystalline U(IV) revealed as major component in uranium ore deposits

Rizlan Bernier-Latmani

Historically, it is believed that crystalline uraninite, produced via the abiotic reduction of hexavalent uranium (U-(VI)) is the dominant reduced U species formed in low-temperature uranium roll-front ore deposits. Here we show that non-crystalline U-(IV) ...

Nature Publishing Group2017

Embrittlement induced by the synergistic effects of radiation damage and helium in structural steels

Kun Wang

Ferritic/martensitic steels are candidate materials for fusion reactor structural components, liquid metal containers of spallation neutron sources, and accelerator driven systems, with good radiation resistance and thermo-mechanical properties. However, e ...

EPFL2015

What Are the Best Materials To Separate a Xenon/Krypton Mixture?

Berend Smit, Cory Matthew Simon, Rocio Mercado, Sondre Kvalvag Schnell

Accelerating progress in the discovery and deployment of advanced nanoporous materials relies on chemical insight and structure-property relationships for rational design. Because of the complexity of this problem, trial-and-error is heavily involved in th ...

American Chemical Society2015

Large eddy simulation of particulate flow inside a differentially heated cavity

Michel Deville, Emmanuel Leriche, Christoph Bosshard, Alfredo Soldati, Abdelouahab Dehbi

In nuclear safety, some severe accident scenarios lead to the presence of fission products in aerosol form in the closed containment atmosphere. It is important to understand the particle depletion process to estimate the risk of a release of radioactivity ...

Elsevier2014