Publications related to Plutonium

Atomic level insight into irradiation effects in nuclear fuel materials

Microstructural evolution during in-pile irradiation, radiation damage effects and fission products behavior in UO2 nuclear fuel are key issues in understanding and for the modeling of the performance as well as safety characteristics of nuclear fuels in t ...

EPFL2024

Design of an Instrumented Fuel Rod for Intra-pin Neutron Flux Measurements in the CROCUS Experimental Reactor

Andreas Pautz, Vincent Pierre Lamirand, Mathieu Hursin, Thomas Jean-François Ligonnet, Won Dong Shin, Tom Mager

In response to the need for validating high-fidelity deterministic neutronics solvers capable of pin-resolved neutron flux distributions, an instrumented fuel rod was designed for the experimental reactor CROCUS, operated by EPFL’s Laboratory for Reactor P ...

2023

Probing Water Dissociation and Oxygen Replacement on Partially Oxygen-Covered Cu(111) by Reflection Absorption Infrared Spectroscopy

Rainer Beck, Mateusz Suchodol, Harmina Vejayan

The presence of chemisorbed oxygen on the Cu(111) surface is known to strongly reduce the activation barrier for water dissociation as compared to bare Cu(111). Here, we present direct experimental evidence for the hydrogen abstraction mechanism responsibl ...

2023

Data-Driven Predictive Models: Calculational Bias in Characterization of Spent Nuclear Fuel

Characteristics of the spent nuclear fuel (SNF) are typically calculated, requiring validation a priori. The validation process relies on the difference between calculations and measurements, namely the bias. Usually, predicting the bias based on benchmark ...

EPFL2022

Investigation and Validation of Unstructured Mesh Methodologies for Modeling Experimental Reactors

Andreas Pautz, Mathieu Hursin, Carlo Fiorina, Tom Mager

This paper summarizes a methodology developed at Ecole Polytechnique Federale de Lausanne for the neutronic modeling of the CROCUS experimental reactor and proposes solutions to the challenges one may face while modeling a research reactor with a complex g ...

MDPI2022

Persistence of the isotopic signature of pentavalent uranium in magnetite

Rizlan Bernier-Latmani, Barbora Bártová, Zezhen Pan

Uranium isotopic signatures can be harnessed to monitor the reductive remediation of subsurface contamination or to reconstruct paleo-redox environments. However, the mechanistic underpinnings of the isotope fractionation associated with U reduction remain ...

2022

On the Capability of Wall-Modeled Large Eddy Simulations to Predict Particle Dispersion in Complex Turbulent Flows

Mohamed Aly Hashem Mohamed Sayed

Predicting particle transport in turbulent flows has a plethora of applications, some of which are: the transport of atmospheric aerosols, the deposition of blood cells in the arteries of human bodies and the atomization of fuel droplets in combustion cham ...

EPFL2022

Design, synthesis, reactivity, and magnetic properties of uranium based oxide and nitride complexes

Luciano Barluzzi

The activation of small molecules is a paramount challenge in modern chemistry. The use of cheap and abundant molecules such as N2, H2, CO2, or CO as energy supplies or as precursors for fine chemicals production is highly desirable. In particular, the onl ...

EPFL2021

Structural performance and mechanical properties investigation of spent nuclear fuel rods under static and dynamic bending loads

Efstathios Vlassopoulos

Currently, most Spent Nuclear Fuel (SNF) is kept safely in storage either at on-site facilities or at centralized interim storage sites. Moreover, many countries face delays in implementing their waste management programmes for SNF and high-level waste dis ...

EPFL2021

Analysis of the first COLIBRI fuel rods oscillation campaign in the CROCUS reactor for the European project CORTEX

Andreas Pautz, Vincent Pierre Lamirand, Mathieu Hursin, Carlo Fiorina, Oskari Ville Pakari, Pavel Frajtag, Axel Guy Marie Laureau, Adolfo Rais, Daniel Godat

The Horizon2020 European project CORTEX aims at developing an innovative core monitoring technique that allows detecting anomalies in nuclear reactors, such as excessive vibrations of core internals, flow blockage, or coolant inlet perturbations. The techn ...

2021

Observation of a singular Weyl point surrounded by charged nodal walls in PtGa

Oleg Yazyev, Jan Hugo Dil, Quansheng Wu, Shengnan Zhang

Constrained by the Nielsen-Ninomiya no-go theorem, in all so-far experimentally determined Weyl semimetals (WSMs) the Weyl points (WPs) always appear in pairs in the momentum space with no exception. As a consequence, Fermi arcs occur on surfaces which con ...

Nature Research2021

Growth and viability of microorganisms in bentonite and their potential activity in deep geological repository environments

Niels Burzan

Radioactive waste is among the most dangerous anthropogenic waste and its safe disposal is a challenging multi-generational task. Many nations have sought for the peaceful application of nuclear fission for the reliable production of electric energy to pow ...

EPFL2021

Preliminary design and analysis of Liquid Fuel Molten Salt Reactor using multi-physics code GeN-Foam

Carlo Fiorina

In this study, a hypothetical fast spectrum Liquid Fuel Molten Salt Reactor (LFMSR) core is modeled using the multiphysics C++ code GeN-Foam (General Nuclear Foam). GeN-Foam is based on OpenFOAM, a C++ opensource library for solution of continuum mechanics ...

ELSEVIER SCIENCE SA2020

Treatment of the implicit effect in Shark-X

Mathieu Hursin, Hakim Ferroukhi, Alexander Vasiliev

Shark-X is a set of Perl-based tools build around the deterministic neutron transport code CASMO-5, used to perform uncertainty quantification for lattice calculations at the Paul Scherrer Institut (PSI). While perturbing an input parameter, e.g. a cross s ...

2020

Data assimilation of post-irradiation examination data for fission yields from GEF

Andreas Pautz, Daniel Jerôme Siefman, Mathieu Hursin, Dimitri Rochman

Nuclear data, especially fission yields, create uncertainties in the predicted concentrations of fission products in spent fuel which can exceed engineering target accuracies. Herein, we present a new framework that extends data assimilation methods to bur ...

EDP SCIENCES S A2020

Data assimilation of post irradiation examination experiments to adjust fission yields

Andreas Pautz, Daniel Jerôme Siefman, Mathieu Hursin

Nuclear data, especially fission yields, create uncertainties in the predicted concentrations of fission products in spent fuel. Herein, we present a new framework that extends data assimilation methods to burnup simulations by using data from post-irradia ...

E D P SCIENCES2020

The shear strength of Opalinus Clay shale in the remoulded state

Alessio Ferrari

The Opalinus Clay shale formation is considered as a potential host geomaterial for the Swiss deep geological repository for radioactive waste. It presents different facies and it is characterised by a multi-scale heterogeneous composition, by a typical fi ...

2020

A mm(3) Fiber-Coupled Scintillator for In-Core Thermal Neutron Detection in CROCUS

Andreas Pautz, Vincent Pierre Lamirand, Oskari Ville Pakari, Pavel Frajtag, Fanny Vitullo, Jean-Baptiste Mosset

This article presents the development, full-characterization, and in-core testing of a miniature neutron detector for the investigation of highly localized in-core neutronics effects in the zero-power reactor CROCUS, operated at the Ecole Polytechnique fed ...

IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC2020

Statistical Burnup Distribution of Moving Pebbles in the High-Temperature Reactor HTR-PM

Andreas Pautz, Jiri Krepel, Fanny Vitullo, Horst-Michael Prasser

In the pebble-bed high-temperature reactor under construction in China, called the HTR-PM, the spherical fuel elements continuously flow downward in the cylindrical core. The burnup of each pebble is checked at the core outlet and, according to the achieve ...

ASME2020

Determination of the activity inventory and associated uncertainty quantification for the CROCUS zero power research reactor

Andreas Pautz, Vincent Pierre Lamirand, Mathieu Hursin, DongHyuk Lee, Pavel Frajtag

The paper describes the source term estimation of CROCUS, the zero power research reactor of EPFL, to be used for dispersion analysis under accidental conditions. To fulfil regulatory requirements, the source term of the CROCUS fuel is estimated through Mo ...

2019