Publications by Quentin Thomas Jeangros

Unveiling the GeI2-Assisted Oriented Growth of Perovskite Crystallite for High-Performance Flexible Sn Perovskite Solar Cells

Tin perovskites are emerging as promising alternatives to their lead-based counterparts for high-performance and flexible perovskite solar cells. However, their rapid crystallization often leads to inadequate film quality and poor device performance. In th ...

2025

Alleviating nanostructural phase impurities enhances the optoelectronic properties, device performance and stability of cesium-formamidinium metal-halide perovskites

Christophe Ballif, Aïcha Hessler-Wyser, Quentin Thomas Jeangros, Beat Ruhstaller, Mostafa Rabie Shlaly Bahr Othman, Daniel Anthony Jacobs, Christian Michael Wolff, Anaël Morgane Jaffrès, Austin George Kuba

The technique of alloying FA+ with Cs+ is often used to promote structural stabilization of the desirable alpha-FAPbI3 phase in halide perovskite devices. However, the precise mechanisms by which these alloying approaches improve the optoelectronic quality ...

Royal Soc Chemistry2024

Linking Nanoscopic Insights to Millimetric-Devices in Formamidinium-Rich Perovskite Photovoltaics

Christophe Ballif, Aïcha Hessler-Wyser, Quentin Thomas Jeangros, Mostafa Rabie Shlaly Bahr Othman

Halide-perovskite semiconductors have a high potential for use in single-junction and tandem solar cells. Despite their unprecedented rise in power conversion efficiencies (PCEs) for photovoltaic (PV) applications, it remains unclear whether perovskite sol ...

Wiley-V C H Verlag Gmbh2024

Synergetic substrate and additive engineering for over 30%-efficient perovskite-Si tandem solar cells

Christophe Ballif, Mounir Driss Mensi, Quentin Thomas Jeangros, Mathieu Gérard Boccard, Daniel Anthony Jacobs, Kerem Artuk, Xin Yu Chin, Deniz Türkay, Christian Michael Wolff

Perovskite-silicon (Si) tandem solar cells are the most prominent contenders to succeed single-junction Si cells that dominate the market today. Yet, to justify the added cost of inserting a perovskite cell on top of Si, these devices should first exhibit ...

2024

Potential-induced degradation in bifacial silicon heterojunction solar modules: Insights and mitigation strategies

Christophe Ballif, Quentin Thomas Jeangros, Alessandro Francesco Aldo Virtuani, Luca Gnocchi, Olatz Arriaga Arruti

Potential-induced degradation (PID) may be a serious concern in photovoltaic (PV) modules and plants, particularly when approaching high system voltages (1500+ V). Here, we investigate PID occurring in bifacial rear-emitter silicon heterojunction (SHJ) sol ...

Wiley2023

Rear textured p-type high temperature passivating contacts and their implementation in perovskite/silicon tandem cells

Christophe Ballif, Antoine Descoeudres, Sylvain Nicolay, Quentin Thomas Jeangros, Philippe Wyss, Soo-Jin Moon, Arnaud Walter, Andrea Ingenito

Silicon solar cells based on high temperature passivating contacts are becoming mainstream in the photovoltaic industry. Here, we developed a high-quality boron-doped poly-silicon hole contact. When combined with a co-processed phosphorus-doped poly-silico ...

Royal Soc Chemistry2023

Operando analysis of a solid oxide fuel cell by environmental transmission electron microscopy

Stefan Diethelm, Aïcha Hessler-Wyser, Jan Van Herle, Quentin Thomas Jeangros, Cédric Frantz

Correlating the microstructure of an energy conversion device to its performance is often a complex exercise, notably in solid oxide fuel cell research. Solid oxide fuel cells combine multiple materials and interfaces that evolve in time due to high operat ...

Nature Portfolio2023

Interface passivation for 31.25%-efficient perovskite/silicon tandem solar cells

Christophe Ballif, Mounir Driss Mensi, Quentin Thomas Jeangros, Mathieu Gérard Boccard, Peter Joseph Fiala, Quentin Jean-Marie Armand Guesnay, Daniel Anthony Jacobs, Kerem Artuk, Xin Yu Chin, Deniz Türkay, Christian Michael Wolff

Silicon solar cells are approaching their theoretical efficiency limit of 29%. This limitation can be exceeded with advanced device architectures, where two or more solar cells are stacked to improve the harvesting of solar energy. In this work, we devise ...

American Association for the Advancement of Science2023

Correlating light-induced deep defects and phase segregation in mixed-halide perovskites

Quentin Thomas Jeangros, Jakub Holovsky, Peter Joseph Fiala, Xin Yu Chin, Christian Michael Wolff

Mixed-halide perovskites are highly promising materials for tandem solar cells. The phenomenon of phase segregation, however hinders their application. Here, we combine Fourier-Transform photocurrent spectroscopy with photoluminescence and current density- ...

Royal Society of Chemistry2022

Monolithic Perovskite-Silicon Tandem Solar Cells: From the Lab to Fab?

Christophe Ballif, Antonin Faes, Quentin Thomas Jeangros, Chien-Jen Yang, Fan Fu

This review focuses on monolithic 2-terminal perovskite-silicon tandem solar cells and discusses key scientific and technological challenges to address in view of an industrial implementation of this technology. The authors start by examining the different ...

Wiley-V C H Verlag Gmbh2022

High-Performance Flexible All-Perovskite Tandem Solar Cells with Reduced V-OC-Deficit in Wide-Bandgap Subcell

Quentin Thomas Jeangros, Cong Chen, Jarla Thiesbrummel, Fan Fu, Xin Yu Chin, Alexander Wieczorek

Among various types of perovskite-based tandem solar cells (TSCs), all-perovskite TSCs are of particular attractiveness for building- and vehicle-integrated photovoltaics, or space energy areas as they can be fabricated on flexible and lightweight substrat ...

WILEY-V C H VERLAG GMBH2022

Three-dimensional in situ imaging of single-grain growth in polycrystalline In2O3:Zr films

Quentin Thomas Jeangros, Michael Elias Stückelberger, Monica Morales Masis

Understanding grain morphology and kinetics of solid-phase crystallization is important for controlling the functional properties of polycrystalline materials. Here, in situ coherent X-ray diffraction imaging and transmission electron microscopy elucidate ...

SPRINGERNATURE2022

Lateral ion migration accelerates degradation in halide perovskite devices

Christophe Ballif, Quentin Thomas Jeangros, Daniel Anthony Jacobs, Kerem Artuk, Xin Yu Chin, Christian Michael Wolff

The migration of mobile ions has long been considered a source of performance degradation in devices based on halide perovskites, but details regarding the mechanisms and extent of this problem remain scarce. Here we report the finding that differences in ...

ROYAL SOC CHEMISTRY2022

Influence of the Dopant Gas Precursor in P-Type Nanocrystalline Silicon Layers on the Performance of Front Junction Heterojunction Solar Cells

Christophe Ballif, Quentin Thomas Jeangros, Mathieu Gérard Boccard, Jean Cattin, Luca Massimiliano Antognini, Mario Joe Lehmann, Vincent Philippe Paratte, Laurie-Lou Senaud, Jan Haschke, Julie Amandine Dreon

Silicon heterojunction solar cells can employ p-type hydrogenated nanocrystalline silicon nc-Si:H(p) on their front side, since these can provide better transparency and contact resistance compared to hydrogenated p-type amorphous silicon layers. We invest ...

2021

Nanoscale Study of the Hole-Selective Passivating Contacts with High Thermal Budget Using C-AFM Tomography

Christophe Ballif, Quentin Thomas Jeangros, Franz-Josef Haug, Gizem Nogay, Martin Ledinsky, Philipp Friedrich Hermann Löper

We investigate hole-selective passivating contacts that consist of an interfacial layer of silicon oxide (SiOx) and a layer of boron-doped SiCx(p). The fabrication process of these contacts involves an annealing step at temperatures above 750 degrees C whi ...

AMER CHEMICAL SOC2021

Evaluation of secondary electron intensities for dopant profiling in ion implanted semiconductors: a correlative study combining SE, SIMS and ECV methods

Aïcha Hessler-Wyser, Quentin Thomas Jeangros, Philippe Wyss, Franz-Josef Haug, Mario Joe Lehmann, Audrey Marie Isabelle Morisset

This study evaluates the secondary electron (SE) dopant contrast in scanning electron microscopy (SEM) and helium ion microscopy (HIM) on boron implanted silicon sample. Complementary techniques like secondary ion mass spectrometry and electrochemical capa ...

IOP PUBLISHING LTD2021

Potential Induced Degradation Mechanism in Rear-Emitter Bifacial Silicon Heterojunction Solar Cells Encapsulated in Different Module Structures

Christophe Ballif, Quentin Thomas Jeangros, Alessandro Francesco Aldo Virtuani, Luca Gnocchi, Olatz Arriaga Arruti

Recent studies showed that silicon heterojunction (SHJ) solar cells can be prone to potential induced degradation (PID) when encapsulated with ethylene vinyl acetate (EVA). Here, to gain understanding in the role of EVA, we perform PID test in humid condit ...

IEEE2021

Vapor deposition of metal halide perovskite thin films: Process control strategies to shape layer properties

Christophe Ballif, Quentin Thomas Jeangros, Florent Sahli, Quentin Jean-Marie Armand Guesnay

Vapor-based processes are particularly promising to deposit the perovskite thin film absorber of solar cells. These deposition methods are up-scalable, involve a controlled solvent-free environment, have the ability to conformally coat rough substrates, in ...

2021

Passivating Polysilicon Recombination Junctions for Crystalline Silicon Solar Cells

Christophe Ballif, Aïcha Hessler-Wyser, Quentin Thomas Jeangros, Philippe Wyss, Franz-Josef Haug, Mario Joe Lehmann, Andrea Ingenito, Audrey Marie Isabelle Morisset

Polysilicon recombination junctions whose n-type bottom layers double as a passivating contact to the silicon surface are investigated. Such recombination junctions are a key element in the interconnection of tandem devices with a silicon bottom cell, and ...

2021

Vapor Transport Deposition of Methylammonium Iodide for Perovskite Solar Cells

Christophe Ballif, Quentin Thomas Jeangros, Cédric Bucher, Florent Sahli, Léo Duchêne, Björn Niesen, Aymeric Michel Schafflützel, Nathanaël Miaz, Quentin Jean-Marie Armand Guesnay, Niccolo Salsi

Vapor-based processes are promising options to deposit metal halide perovskite solar cells in an industrial environment due to their ability to deposit uniform layers over large areas in a controlled environment without resorting to the use of (possibly to ...

2021