Publications by Han-Hee Cho | EPFL Graph Search

Decoupling Interlayer Spacing and Cation Dipole on Exciton Binding Energy in Layered Halide Perovskites

Rosario Scopelliti, Nicolas Grandjean, Jun Ho Yum, Kevin Sivula, Simon Nussbaum, Han-Hee Cho, Yeonju Kim

Layered halide perovskites (LHPs) are emerging semiconductor materials due to their superior environmental stability compared to that of traditional halide perovskites. While LHPs have tunable optoelectronic properties, quantum and dielectric confinement e ...

2024

Assessing the Charge Carrier Dynamics at Hybrid Interfaces of Organic Photoanodes for Solar Fuels

Kevin Sivula, Yongpeng Liu, Han-Hee Cho, Alexander Wieczorek

Organic semiconductors (OSCs) have emerged as promising active layers for photoanodes to drive photoelectrochemical (PEC) oxidation reactions. Interfacing an OSC with an inorganic electron transport layer (ETL) is key to enabling both high performance and ...

Amer Chemical Soc2024

An Organic Semiconductor Photoelectrochemical Tandem Cell for Solar Water Splitting

Mounir Driss Mensi, Jun Ho Yum, Kevin Sivula, Han-Hee Cho, Dan Zhang

Photoelectrochemical cells employing organic semiconductors (OS) are promising for solar-to-fuel conversion via water splitting. However, despite encouraging advances with the half reactions, complete overall water splitting remains a challenge. Herein, a ...

WILEY-V C H VERLAG GMBH2022

Bulk Heterojunction Organic Semiconductor Photoanodes: Tuning Energy Levels to Optimize Electron Injection

Jun Ho Yum, Kevin Sivula, Nestor Guijarro Carratala, Arvindh Sekar, Liang Yao, Barbara Alexandra Primera Darwich, Yongpeng Liu, Han-Hee Cho, Juan Manuel Moreno Naranjo

The use of a bulk heterojunction of organic semiconductors to drive photoelectrochemical water splitting is an emerging trend; however, the optimum energy levels of the donor and acceptor have not been established for photoanode operation with respect to e ...

AMER CHEMICAL SOC2022

Benzodithiophene‐Based Spacers for Layered and Quasi‐Layered Lead Halide Perovskite Solar Cells

Mounir Driss Mensi, Jun Ho Yum, Kevin Sivula, Nestor Guijarro Carratala, Luc Emile Monnier, Liang Yao, Barbara Alexandra Primera Darwich, Han-Hee Cho

Incorporating extended pi-conjugated organic cations in layered lead halide perovskites is a recent trend promising to merge the fields of organic semiconductors and lead halide perovskites. Herein, we integrate benzodithiophene (BDT) into Ruddlesden–Poppe ...

2021

A semiconducting polymer bulk heterojunction photoanode for solar water oxidation

Jun Ho Yum, Kevin Sivula, Nestor Guijarro Carratala, Arvindh Sekar, Liang Yao, Yongpeng Liu, Rebekah Anne Wells, Florent Alexandre Boudoire, Han-Hee Cho

Organic semiconductors hold promise to enable scalable, low-cost and high-performance artificial photosynthesis. However, the performance of systems based on organic semiconductors for light-driven water oxidation have remained poor compared with inorganic ...

NATURE RESEARCH2021

A hybrid bulk-heterojunction photoanode for direct solar-to-chemical conversion dagger

Michael Graetzel, Jun Ho Yum, Kevin Sivula, Nestor Guijarro Carratala, Arvindh Sekar, Liang Yao, Barbara Alexandra Primera Darwich, Yongpeng Liu, Rebekah Anne Wells, Dan Ren, Han-Hee Cho, Meng Xia

Organic semiconductors (OSs) are emerging candidates as light-harvesting materials in photoelectrochemical (PEC) cells for direct solar-to-chemical conversion. Despite significant recent progress with OS-based photocathodes, the development of efficient an ...

ROYAL SOC CHEMISTRY2021

Establishing Stability in Organic Semiconductor Photocathodes for Solar Hydrogen Production

Jun Ho Yum, Kevin Sivula, Florian Le Formal, Muhammad Aiman Bin Rahmanudin Hamdan, Nestor Guijarro Carratala, Arvindh Sekar, Liang Yao, Yongpeng Liu, Rebekah Anne Wells, Florent Alexandre Boudoire, Han-Hee Cho

As organic semiconductors attract increasing attention to application in the fields of bioelectronics and artificial photosynthesis, understanding the factors that determine their robust operation in direct contact with aqueous electrolytes becomes a criti ...

AMER CHEMICAL SOC2020

Fully Conjugated Donor–Acceptor Block Copolymers for Organic Photovoltaics via Heck–Mizoroki Coupling

Kevin Sivula, Arvindh Sekar, Liang Yao, Yongpeng Liu, Charles Roger Jean Lhermitte, Han-Hee Cho

2019

Lead Halide Perovskite Quantum Dots to Enhance the Power Conversion Efficiency of Organic Solar Cells

Jun Ho Yum, Kevin Sivula, Florian Le Formal, Nestor Guijarro Carratala, Liang Yao, Barbara Alexandra Primera Darwich, Yongpeng Liu, Rebekah Anne Wells, Lucie Navratilova, Han-Hee Cho

The facile synthesis, solution-processability, and outstanding optoelectronic properties of emerging colloidal lead halide perovskite quantum dots (LHP QDs) makes them ideal candidates for scalable and inexpensive optoelectronic applications, including pho ...

Wiley-VCH Verlag GmbH2019

Multiarm and Substituent Effects on Charge Transport of Organic Hole Transport Materials

Mohammad Khaja Nazeeruddin, Kevin Sivula, Antonio Prlj, Nikita Drigo, Liang Yao, Kun-Han Lin, Han-Hee Cho

We explore several potential dopant-free triphenylamine-based hole transport materials for perovskite solar cells by combining two design strategies: (1) incorporation of multiple arms for mobility enhancement and (2) including Lewis bases that assist in d ...

2019