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Christian Michael Wolff

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Related publications (33)

A Universal Perovskite/C60 Interface Modification via Atomic Layer Deposited Aluminum Oxide for Perovskite Solar Cells and Perovskite-Silicon Tandems

Christophe Ballif, Aïcha Hessler-Wyser, Mounir Driss Mensi, Mostafa Rabie Shlaly Bahr Othman, Kerem Artuk, Deniz Türkay, Christian Michael Wolff

The primary performance limitation in inverted perovskite-based solar cells is the interface between the fullerene-based electron transport layers and the perovskite. Atomic layer deposited thin aluminum oxide (AlOX) interlayers that reduce nonradiative re ...

Wiley-V C H Verlag Gmbh2024

Blade-Coating of High Crystallinity Cesium-Formamidinium Perovskite Formulations

Christophe Ballif, Aïcha Hessler-Wyser, Mostafa Rabie Shlaly Bahr Othman, Christian Michael Wolff, Anaël Morgane Jaffrès

Up-scalable coating processes need to be developed to manufacture efficient and stable perovskite-based solar modules. In this work, we combine two Lewis base additives (N,N′-dimethylpropyleneurea and thiourea) to fabricate high-quality Cs0.15FA0.85PbI3 pe ...

2024

Improving the photo-stability of triple cation perovskite solar cells using chromophore-infused optically transparent Pectin/polymethyl methacrylate composite

Christophe Ballif, Aïcha Hessler-Wyser, Mostafa Rabie Shlaly Bahr Othman, Christian Michael Wolff

Perovskite solar cells (PSCs) show great promise due to their high efficiency and low manufacturing costs, yet they encounter notable challenges such as optical losses and stability issues, mainly due to high surface reflection and degradation from UV irra ...

FUNDACIO DE LA COMUNITAT VALENCIANA SCITO2024

Perovskite/Silicon Tandem Solar Cells Above 30% Conversion Efficiency on Submicron-Sized Textured Czochralski-Silicon Bottom Cells with Improved Hole-Transport Layers

Christophe Ballif, Kerem Artuk, Christian Michael Wolff

In perovskite/silicon tandem solar cells, the utilization of silicon heterojunction (SHJ) solar cells as bottom cells is one of the most promising concepts. Here, we present optimization strategies for the top cell processing and their integration into SHJ ...

2024

Alleviating nanostructural phase impurities enhances the optoelectronic properties, device performance and stability of cesium-formamidinium metal-halide perovskites

Christophe Ballif, Aïcha Hessler-Wyser, Quentin Thomas Jeangros, Beat Ruhstaller, Mostafa Rabie Shlaly Bahr Othman, Daniel Anthony Jacobs, Christian Michael Wolff, Anaël Morgane Jaffrès, Austin George Kuba

The technique of alloying FA+ with Cs+ is often used to promote structural stabilization of the desirable alpha-FAPbI3 phase in halide perovskite devices. However, the precise mechanisms by which these alloying approaches improve the optoelectronic quality ...

Royal Soc Chemistry2024

Understanding and Mitigating the Degradation of Perovskite Solar Cells Based on a Nickel Oxide Hole Transport Material during Damp Heat Testing

Christophe Ballif, Mounir Driss Mensi, Jun Ho Yum, Kevin Sivula, Yongpeng Liu, Marion Solange Madeleine Dussouillez, Christian Michael Wolff

The development of stable materials, processable on alarge area,is a prerequisite for perovskite industrialization. Beyond the perovskiteabsorber itself, this should also guide the development of all otherlayers in the solar cell. In this regard, the use o ...

AMER CHEMICAL SOC2023

Interface passivation for 31.25%-efficient perovskite/silicon tandem solar cells

Christophe Ballif, Mounir Driss Mensi, Quentin Thomas Jeangros, Mathieu Gérard Boccard, Peter Joseph Fiala, Quentin Jean-Marie Armand Guesnay, Daniel Anthony Jacobs, Kerem Artuk, Xin Yu Chin, Deniz Türkay, Christian Michael Wolff

Silicon solar cells are approaching their theoretical efficiency limit of 29%. This limitation can be exceeded with advanced device architectures, where two or more solar cells are stacked to improve the harvesting of solar energy. In this work, we devise ...

American Association for the Advancement of Science2023

Rationalizing Performance Losses of Wide Bandgap Perovskite Solar Cells Evident in Data from the Perovskite Database

Tor Jesper Jacobsson, Christian Michael Wolff

Metal halide perovskites (MHPs) have become a widely studied class of semiconductors for various optoelectronic devices. The possibility to tune their bandgap (E-g) over a broad spectral range from 1.2 eV to 3 eV by compositional engineering makes them par ...

Wiley-V C H Verlag Gmbh2023

Lateral ion migration accelerates degradation in halide perovskite devices

Christophe Ballif, Quentin Thomas Jeangros, Daniel Anthony Jacobs, Kerem Artuk, Xin Yu Chin, Christian Michael Wolff

The migration of mobile ions has long been considered a source of performance degradation in devices based on halide perovskites, but details regarding the mechanisms and extent of this problem remain scarce. Here we report the finding that differences in ...

ROYAL SOC CHEMISTRY2022

Correlating light-induced deep defects and phase segregation in mixed-halide perovskites

Quentin Thomas Jeangros, Jakub Holovsky, Peter Joseph Fiala, Xin Yu Chin, Christian Michael Wolff

Mixed-halide perovskites are highly promising materials for tandem solar cells. The phenomenon of phase segregation, however hinders their application. Here, we combine Fourier-Transform photocurrent spectroscopy with photoluminescence and current density- ...

Royal Society of Chemistry2022

Laser Patterned Flexible 4T Perovskite-Cu(In,Ga)Se-2 Tandem Mini-module with Over 18% Efficiency

Kerem Artuk, Christian Michael Wolff

Perovskite-Cu(In,Ga)Se-2 (CIGS) thin-film tandem technology provides an exciting prospect to achieve low-cost high-efficiency photovoltaic devices by high throughput roll-to-roll processing on flexible substrates. However, no report on flexible perovskite- ...

WILEY-V C H VERLAG GMBH2022

Nano-emitting Heterostructures Violate Optical Reciprocity and Enable Efficient Photoluminescence in Halide-Segregated Methylammonium-Free Wide Bandgap Perovskites

Christophe Ballif, Quentin Thomas Jeangros, Peter Joseph Fiala, Chien-Jen Yang, Pietro Caprioglio, Christian Michael Wolff

This work investigates halide segregation in methylammonium-free wide bandgap perovskites by photoluminescence quantum yield (PLQY) and advanced electron microscopy techniques. Our study reveals how the formation of nano-emitting low-energy domains embedde ...

AMER CHEMICAL SOC2021

Bi-functional interfaces by poly(ionic liquid) treatment in efficient pin and nip perovskite solar cells

Mohammad Khaja Nazeeruddin, Antonio Abate, Giulia Grancini, Filippo de Angelis, Albertus Adrian Sutanto, Pietro Caprioglio, Christian Michael Wolff

Approaches to boost the efficiency and stability of perovskite solar cells often address one singular problem in a specific device configuration. In this work, we utilize a poly(ionic liquid) (PIL) to introduce a multi-functional interlayer to improve the ...

ROYAL SOC CHEMISTRY2021

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