Publications by Andrea Baccarini

Atmospheric reactive nitrogen and its dry deposition regimes under anthropogenic influence: Insights from intensive and long-term monitoring in Switzerland

Athanasios Nenes, Kalliopi Violaki, Ghislain Gilles Jean-Michel Motos, Andrea Baccarini

Excessive nitrogen deposition from anthropogenic activities poses significant challenges to ecosystems and air quality.1 The atmospheric deposition of ammonium and nitrate plays a critical role in regulating ecosystem productivity and driving particulate m ...

2025

Observations of high-time-resolution and size-resolved aerosol chemical composition and microphysics in the central Arctic: implications for climate-relevant particle properties

Benjamin Jérémy Laurent Heutte, Julia Schmale, Ivo Fabio Beck, Andrea Baccarini, Lubna Dada, Hélène Paule Angot, Jakob Boyd Pernov, Nora Bergner, Markus Frey

Aerosols play a critical role in the Arctic's radiative balance, influencing solar radiation and cloud formation. Limited observations in the central Arctic leave gaps in understanding aerosol dynamics year-round, affecting model predictions of climate-rel ...

Copernicus GmbH2025

Investigating processes influencing simulation of local Arctic wintertime anthropogenic pollution in Fairbanks, Alaska, during ALPACA-2022

Roman Pohorsky, Julia Schmale, Andrea Baccarini

Lagrangian tracer simulations are deployed to investigate processes influencing vertical and horizontal dispersion of anthropogenic pollution in Fairbanks, Alaska, during the Alaskan Layered Pollution and Chemical Analysis (ALPACA) 2022 field campaign. Sim ...

Copernicus GmbH2025

Anthropogenic organic aerosol in Europe produced mainly through second-generation oxidation

Andrea Baccarini

Exposure to anthropogenic atmospheric aerosol is a major health issue, causing several million deaths per year worldwide. The oxidation of aromatic hydrocarbons from traffic and wood combustion is an important anthropogenic source of low-volatility species ...

NATURE PORTFOLIO2025

Surface distributions and vertical profiles of trace gases (CO, O3, NO, NO2) in the Arctic wintertime boundary layer using low-cost sensors during ALPACA-2022

Roman Pohorsky, Julia Schmale, Andrea Baccarini

Electrochemical gas sensors (EGSs) have been used to measure the surface distributions and vertical profiles of trace gases in the wintertime Arctic boundary layer during the Alaskan Layered Pollution and Chemical Analysis (ALPACA) field experiment in Fair ...

COPERNICUS GESELLSCHAFT MBH2025

In situ vertical observations of the layered structure of air pollution in a continental high-latitude urban boundary layer during winter

Roman Pohorsky, Julia Schmale, Andrea Baccarini

Vertical in situ measurements of aerosols and trace gases were conducted in Fairbanks, Alaska, during winter 2022 as part of the Alaskan Layered Pollution and Chemical Analysis campaign (ALPACA). Using a tethered balloon, the study explores the dispersion ...

Copernicus GmbH2025

Temperature, humidity, and ionisation effect of iodine oxoacid nucleation

Andrea Baccarini, Lubna Dada, Houssni Lamkaddam, Imad El Haddad

Iodine oxoacids are recognised for their significant contribution to the formation of new particles in marine and polar atmospheres. Nevertheless, to incorporate the iodine oxoacid nucleation mechanism into global simulations, it is essential to comprehend ...

Royal Soc Chemistry2024

Highly Hygroscopic Aerosols Facilitate Summer and Early‐Autumn Cloud Formation at Extremely Low Concentrations Over the Central Arctic Ocean

Julia Schmale, Andrea Baccarini

Arctic clouds are sensitive to atmospheric particles since these are sometimes in such low concentrations that clouds cannot always form under supersaturated water vapor conditions. This is especially true in the late summer, when aerosol concentrations ar ...

2024

Equivalent black carbon concentration measured with an aethalometer AE33 during the Arctic Ocean 2018 expedition

Benjamin Jérémy Laurent Heutte, Julia Schmale, Andrea Baccarini

Equivalent black carbon (eBC) mass concentration was measured with a commercial aethalometer (model AE33, Magee Scientific, Berkeley, USA). Measurements were performed onboard of the Swedish icebreaker (I/B) Oden from August to September 2018 as part of th ...

EPFL Infoscience2024

Overview of the Alaskan Layered Pollution and Chemical Analysis (ALPACA) Field Experiment

Roman Pohorsky, Julia Schmale, Athanasios Nenes, Sukriti Kapur, Andrea Baccarini

The Alaskan Layered Pollution And Chemical Analysis (ALPACA) field experiment was a collaborative study designed to improve understanding of pollution sources and chemical processes during winter (cold climate and low-photochemical activity), to investigat ...

2024

Atmospheric isoprene measurements reveal larger-than-expected Southern Ocean emissions

Julia Schmale, Andrea Baccarini

Isoprene is a key trace component of the atmosphere emitted by vegetation and other organisms. It is highly reactive and can impact atmospheric composition and climate by affecting the greenhouse gases ozone and methane and secondary organic aerosol format ...

Nature Research2024

Modular Multiplatform Compatible Air Measurement System (MoMuCAMS): a new modular platform for boundary layer aerosol and trace gas vertical measurements in extreme environments

Roman Pohorsky, Julia Schmale, Andrea Baccarini

The Modular Multiplatform Compatible Air Measurement System (MoMuCAMS) is a newly developed in situ aerosol and trace gas measurement platform for lower-atmospheric vertical profiling. MoMuCAMS has been primarily designed to be attached to a Helikite, a ru ...

2024

MoMuCAMS: A new modular platform for boundary layer aerosol and trace gas vertical measurements in extreme environments

Roman Pohorsky, Julia Schmale, Andrea Baccarini

The Modular Multiplatform Compatible Air Measurement System (MoMuCAMS) is a newly developed in situ aerosol and trace gas measurement payload for lower atmospheric vertical profiling in extreme environments. MoMuCAMS is a multiplatform compatible system, p ...

2023

Iodine oxoacids enhance nucleation of sulfuric acid particles in the atmosphere

Andrea Baccarini, Lubna Dada, André Welti, Houssni Lamkaddam, Imad El Haddad, Mihnea Surdu

The main nucleating vapor in the atmosphere is thought to be sulfuric acid (H2SO4), stabilized by ammonia (NH3). However, in marine and polar regions, NH3 is generally low, and H2SO4 is frequently found together with iodine oxoacids [HIOx, i.e., iodic acid ...

American Association for the Advancement of Science2023

Role of sesquiterpenes in biogenic new particle formation

Federico Bianchi, Andrea Baccarini, Lubna Dada, Imad El Haddad

Biogenic vapors form new particles in the atmosphere, affecting global climate. The contributions of monoterpenes and isoprene to new particle formation (NPF) have been extensively studied. However, sesquiterpenes have received little attention despite a p ...

2023

Late summer transition from a free-tropospheric to boundary layer source of Aitken mode aerosol in the high Arctic

Julia Schmale, Andrea Baccarini

Copernicus Publications2023

Pollution mask for the continuous corrected particle number concentration data in 1 min time resolution measured in the Swiss aerosol container using a whole air inlet during MOSAiC 2019/2020

Julia Schmale, Ivo Fabio Beck, Andrea Baccarini, Hélène Paule Angot

This dataset contains particle number concentrations and a pollution flag in 1 min time resolution. It is derived by the pollution detection algorithm (PDA, doi:10.5281/zenodo.5761101) based on the corrected particle number concentration data of the CPC377 ...

Zenodo2023

Pollution mask for the continuous corrected particle number concentration data in 1 min resolution, measured in the Swiss aerosol container during MOSAiC 2019/2020

Julia Schmale, Ivo Fabio Beck, Andrea Baccarini, Hélène Paule Angot

This dataset contains a pollution flag in 1 min time resolution. It is derived by the pollution detection algorithm (PDA) based on the corrected particle number concentration data (DOI upcoming) measured during the year long MOSAiC expedition from October ...

Zenodo2022

Physical and Chemical Properties of Cloud Droplet Residuals and Aerosol Particles During the Arctic Ocean 2018 Expedition

Julia Schmale, Andrea Baccarini, Lubna Dada

Detailed knowledge of the physical and chemical properties and sources of particles that form clouds is especially important in pristine areas like the Arctic, where particle concentrations are often low and observations are sparse. Here, we present in sit ...

2022

The gas-phase formation mechanism of iodic acid as an atmospheric aerosol source

Andrea Baccarini

Iodine is a reactive trace element in atmospheric chemistry that destroys ozone and nucleates particles. Iodine emissions have tripled since 1950 and are projected to keep increasing with rising O-3 surface concentrations. Although iodic acid (HIO3) is wid ...

NATURE PORTFOLIO2022