Publication

Isobaric production cross sections from 0.6 GeV proton irradiation of neptunium and thorium using mass spectrometry

Rakesh Chawla
2006
Journal Articles

Abstract

A high-fluence proton irradiation of neptunium was the last experiment in PSIs programme ATHENA related to accelerator-based transmutation. The principal aim of the programme has been to provide experimental data for the validation of theoretical models in nucleon-meson transport codes, with emphasis on the mass yield distribution of fission and spallation products. An improved mass spectrometry method has allowed the direct derivation of isobaric production cross sections with only minor corrections and an estimate of the fission cross section by integration in the fission hump. In a second sample position of the irradiation head, a repetition of the previous ATHENA experiment with thorium was possible, profiting from the improved mass spectrometry technique. The experimental results are better predicted by the code FUSSPOT than by HETC/RAL, both used at PSI. [All rights reserved Elsevier]

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https://infoscience.epfl.ch/entities/publication/d5c2a78a-fcf8-48e9-9ff8-a7cb3f95a1e6

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Rakesh Chawla
2006
Journal Articles

Abstract

Official source

https://infoscience.epfl.ch/entities/publication/d5c2a78a-fcf8-48e9-9ff8-a7cb3f95a1e6

About this result

Ontological neighbourhood

Energy engineering

Nuclear power: Topics in nuclear power

Related concepts (32)

Mass spectrometry

Mass spectrometry (MS) is an analytical technique that is used to measure the mass-to-charge ratio of ions. The results are presented as a mass spectrum, a plot of intensity as a function of the mass-to-charge ratio. Mass spectrometry is used in many different fields and is applied to pure samples as well as complex mixtures. A mass spectrum is a type of plot of the ion signal as a function of the mass-to-charge ratio.

Ion-mobility spectrometry–mass spectrometry

Ion mobility spectrometry–mass spectrometry (IMS-MS) is an analytical chemistry method that separates gas phase ions based on their interaction with a collision gas and their masses. In the first step, the ions are separated according to their mobility through a buffer gas on a millisecond timescale using an ion mobility spectrometer. The separated ions are then introduced into a mass analyzer in a second step where their mass-to-charge ratios can be determined on a microsecond timescale.

Nuclear fission

Nuclear fission is a reaction in which the nucleus of an atom splits into two or more smaller nuclei. The fission process often produces gamma photons, and releases a very large amount of energy even by the energetic standards of radioactive decay. Nuclear fission was discovered on 19 December 1938 in Berlin by German chemists Otto Hahn and Fritz Strassmann. Physicists Lise Meitner and her nephew Otto Robert Frisch explained it theoretically in January 1939. Frisch named the process "fission" by analogy with biological fission of living cells.

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