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Publications associées (31)

Photoelectrochemical Oxygen Evolution on Mesoporous Hematite Films Prepared from Maghemite Nanoparticles

Michael Graetzel, Shaik Mohammed Zakeeruddin, Nathália Carolina Verissimo

Iron oxides, especially hematite (alpha-Fe2O3), a are promising materials for applications in photoelectrochemical cells and photo-redox catalysis. However, realizing high-performance hematite photoanodes via an environmentally-friendly route remains a gre ...

2022

Modeling the Photostability of Solar Water-Splitting Devices and Stabilization Strategies

Sophia Haussener, Fredy Intelligent Nandjou Dongmeza

The practical implementation of photoelectrochemical devices for hydrogen generation is limited by their short lifetimes. Understanding the factors affecting the stability of the heterogeneous photoelectrodes is required to formulate degradation mitigation ...

2022

Multiple Effects Induced by Mo6+ Doping in BiVO4 Photoanodes

Kevin Sivula, Charles Roger Jean Lhermitte, Nukorn Plainpan, Annalisa Polo, Ivan Grigioni

Mo6+ doping increases the photoelectrochemical performance of BiVO4 photoanodes in water oxidation. Herein, the underlying mechanisms is elucidated through a systematic structural, morphological, and photoelectrochemical investigation on photoelectrodes of ...

WILEY-V C H VERLAG GMBH2022

Derivative voltammetry: a simple tool to probe reaction selectivity in photoelectrochemical cells

Kevin Sivula, Florent Alexandre Boudoire, Nukorn Plainpan

We demonstrate the use of the derivative voltammogram method to predict the selectivity of the photo-driven oxidation of 5-hydroxymethylfurfural (HMF) on a WO3 photoanode as a function of applied potential using only information obtained from the linear sw ...

2022

Photo‐Electrochemical Conversion of CO 2 Under Concentrated Sunlight Enables Combination of High Reaction Rate and Efficiency

Sophia Haussener, Etienne Boutin, Mahendra Patel, Silvan Suter

Photo-electrochemical production of solar fuels from carbon dioxide, water, and sunlight is an appealing approach. Nevertheless, it remains challenging to scale despite encouraging demonstrations at low power input. Higher current densities require notable ...

Wiley2022

Solar fuel processing: Comparative mini-review on research, technology development, and scaling

Sophia Haussener

Solar energy provides an unprecedented potential as a renewable and sustainable energy resource and will substantially reshape our future energy economy. It is not only useful in producing electricity but also (high-temperature) heat and fuel, both require ...

2022

Organic Semiconductors For Photoelectrochemical Applications

Arvindh Sekar

The capture and conversion of solar energy into other useful forms has been the topic of discussion for the past few decades, accentuated by the need to combat climate change and face the challenge of non-renewability of conventional sources of fuel for ou ...

EPFL2022

Modeling and assessment of high-temperature photo-electrochemical devices

Ronald Ramiro Gutierrez Perez

In this thesis, the feasibility and performance of photo-driven electrochemical (PEC) devices working at elevated temperatures (T>700 K) is investigated and modeled. In such high-temperature PEC devices, a part of the solar spectrum is used for generating ...

EPFL2022

Photochemical oxidation of phenols and anilines mediated by phenoxyl radicals in aqueous solution

Urs von Gunten, Silvio Canonica, Stephanie Christa Remke

Reactive intermediates formed upon irradiation of chromophoric dissolved organic matter (CDOM) contribute to the degradation of various organic contaminants in surface waters. Besides well-studied "short-lived" photo oxidants, such as triplet state CDOM (3 ...

PERGAMON-ELSEVIER SCIENCE LTD2022

Water photo-oxidation on self-assembled organic/Co3O4 metal junctions in biphasic systems

Hubert Girault, Astrid Johana Olaya Avendano, Julieta Soledad Riva

A microwater vertical bar butyronitrile (W vertical bar BCN) interface was used to study the effect of the interfacial chemical polarization on the efficiency of the visible-light induced water oxidation reaction (WOR) by the electron acceptor/ photosensit ...

PERGAMON-ELSEVIER SCIENCE LTD2022

Solar water purification with photocatalytic nanocomposite filter based on TiO2 nanowires and carbon nanotubes

László Forró, Luca Rossi, Andrzej Sienkiewicz, Endre Horvath, Florian Frédéric Vincent Breider, Dominique Grandjean, Miriam Gaál

Water contamination due to environmental conditions and poor waste management in certain areas of the world represents a serious problem in accessing clean and safe drinking water. This problem is especially critical in electricity-poor regions, where adva ...

2022

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