Publications associées à Smog

Overview of the Alaskan Layered Pollution and Chemical Analysis (ALPACA) Field Experiment

Athanasios Nenes, Julia Schmale, Andrea Baccarini, Roman Pohorsky, Sukriti Kapur

The Alaskan Layered Pollution And Chemical Analysis (ALPACA) field experiment was a collaborative study designed to improve understanding of pollution sources and chemical processes during winter (cold climate and low-photochemical activity), to investigat ...

2024

Nitrogen oxides in the free troposphere: implications for tropospheric oxidants and the interpretation of satellite NO2 measurements

Ilann Ernest Valentin Bourgeois

Satellite-based retrievals of tropospheric NO(2)columns are widely used to infer NOx (equivalent to NO + NO2) emissions. These retrievals rely on model information for the vertical distribution of NO2. The free tropospheric background above 2 km is particu ...

Copernicus GmbH2023

One-pot synthesis of highly dispersed mesoporous Cu/ZrO2 catalysts for NH3-SCR

Oliver Kröcher, Davide Ferri, Rob Jeremiah G. Nuguid

Catalysts consisting of highly dispersed copper on a mesoporous ZrO2 support were synthesised via a one-pot sol-gel synthesis and were tested for the selective catalytic reduction of NOx by NH3. The copper dispersion was investigated by XRD and TEM, which ...

ELSEVIER2022

Year-long variability of polycyclic aromatic hydrocarbons (PAHs) and their contribution on winter intense pollution events in the urban environment of Athens, Greece

Athanasios Nenes, Maria Apostolaki

Polycyclic aromatic hydrocarbons (PAHs) are organic pollutants with proven mutagenic and carcinogenic potential that originate from incomplete combustion, and partition to fine particulate matter. Nitro-PAHs & oxy-PAHs are oxidation products of PAHs with i ...

2021

Nighttime chemistry of biomass burning emissions in urban areas: A dual mobile chamber study

Athanasios Nenes, Spyros Pandis

Residential biomass burning for heating purposes is an important source of air pollutants during winter. Here we test the hypothesis that significant secondary organic aerosol production can take place even during winter nights through oxidation of the emi ...

Copernicus GmbH2021

Historical Changes in Seasonal Aerosol Acidity in the Po Valley (Italy) as Inferred from Fog Water and Aerosol Measurements

Athanasios Nenes, Spyros Pandis

Acidity profoundly affects almost every aspect that shapes the composition of ambient particles and their environmental impact. Thermodynamic analysis of gas-particle composition datasets offers robust estimates of acidity, but they are not available for l ...

AMER CHEMICAL SOC2021

Rapid dark aging of biomass burning as an overlooked source of oxidized organic aerosol

Athanasios Nenes, Spyros Pandis

Oxidized organic aerosol (OOA) is a major component of ambient particulate matter, substantially impacting climate, human health, and ecosystems. OOA is readily produced in the presence of sunlight, and requires days of photooxidation to reach the levels o ...

National Academy of Sciences2020

Exploring chemical space in the search for improved azoheteroarene-based photoswitches

Anne-Clémence Corminboeuf, Sergio Vela Llausi

In quest of improved photo switches, azoheteroarenes have emerged as a potential alternative to azobenzenes. However, to date the number and types of these species that have been subjected to study are insufficient to provide an in-depth understanding of t ...

ROYAL SOC CHEMISTRY2019

Photosensitizing and Inhibitory Effects of Ozonated Dissolved Organic Matter on Triplet-Induced Contaminant Transformation

Urs von Gunten, Silvio Canonica

Dissolved organic matter (DOM) is both a promoter and an inhibitor of triplet-induced organic contaminant oxidation. This dual role was systematically investigated through photochemical experiments with three types of DOM of terrestrial and aquatic origins ...

American Chemical Society2015

Impact of Operating Regime on Aviation Engine Emissions: Modeling Study

Pénélope Leyland

This work is focused on the numerical analysis of pollutant formation in an aviation gas turbine engine at different values of power setting. The analysis is conducted on the basis of a comprehensive approach treating the reactor net model for description ...

Amer Inst Aeronautics Astronautics2013

Impacts of changes in land use and land cover on atmospheric chemistry and air quality over the 21st century

Jed Oliver Kaplan, Songmei Wu

The effects of future land use and land cover change on the chemical composition of the atmosphere and air quality are largely unknown. To investigate the potential effects associated with future changes in vegetation driven by atmospheric CO2 concentratio ...

Copernicus Publications2012

The influence of foreign vs. North American emissions on surface ozone in the US

As part of the Hemispheric Transport of Air Pollution (HTAP; < a href='http://www.htap.org' target='_blank'> http:// www.htap.org ) project, we analyze results from 15 global and 1 hemispheric chemical transport models and compare these to Clean Air S ...

Copernicus Publications2009

Interannual variability in tropospheric ozone and its precursors : a modeling study constrained by long-term ground-based and satellite observations

Symeon Koumoutsaris

Tropospheric ozone (O3) is a harmful pollutant and an increasingly important green-house gas. Tropospheric O3 distributions are determined by complex and non-linear interactions between photochemistry and transport processes. The first objective of this th ...

EPFL2008

A model investigation of tropospheric ozone chemical tendencies in long-range transported pollution plumes

Isabelle Bey, Marion Auvray

The impact of continental outflow on the ozone chemical tendencies (i.e., production and loss rates) is quantified in the North Atlantic and northwest Pacific regions using the GEOS-Chem and the MOZECH global models of chemistry and transport. The ozone te ...

2007

Improvement of an urban turbulence parametrization for meteorological operational forecast and air quality modeling

Clive Muller

During the last century, urban pollution has increased with the growth of cities. Urban air quality has become a high priority as it is directly linked to concerns such as human exposure and health. The present work is dedicated to urban air quality modeli ...

EPFL2007

Long-range transport of pollution to Europe : origins, chemical and transport pathways, and impact on tropospheric composition

Marion Auvray

Ozone (O3) and aerosols are harmful to human health. Long-range transport sources contribute to the background levels upon which local pollution builds. The goal of this thesis is to describe and quantify the respective contribution of local and long-range ...

EPFL2006

Long-Range Transport to Europe : Seasonal Variations and Implications for the European Ozone Budget

Isabelle Bey, Marion Auvray

We use a chemical transport model (GEOS-CHEM) to quantify the contribution of long-range transported pollution to the European ozone ({O}{3}) budget for the year 1997. The model reproduces the main features observed over Europe for {O}{3}, carbon monoxid ...

2005

Estimation of the total VOC reactivity with OH by pump-and-probe OH lidar to determine a new indicator for ozone production

Many of our most severe problems of environmental pollution involve the Earth's atmosphere. The adverse effects of atmospheric pollution are particularly evident in the low troposphere, especially in urban/suburban areas where many sources contribute to th ...

EPFL2000