Publications associées à Assombrissement global

Implementation of the ISORROPIA-lite aerosol thermodynamics model into the EMAC chemistry climate model (based on MESSy v2.55): implications for aerosol composition and acidity

This study explores the differences in performance and results by various versions of the ISORROPIA thermodynamic module implemented within the ECHAM/MESSy Atmospheric Chemistry (EMAC) model. Three different versions of the module were used, ISORROPIA II v ...

Copernicus Gesellschaft Mbh2024

Role of sesquiterpenes in biogenic new particle formation

Andrea Baccarini, Imad El Haddad, Lubna Dada, Federico Bianchi

Biogenic vapors form new particles in the atmosphere, affecting global climate. The contributions of monoterpenes and isoprene to new particle formation (NPF) have been extensively studied. However, sesquiterpenes have received little attention despite a p ...

2023

Reducing Aerosol Forcing Uncertainty by Combining Models With Satellite and Within-The-Atmosphere Observations: A Three-Way Street

Athanasios Nenes

Aerosol forcing uncertainty represents the largest climate forcing uncertainty overall. Its magnitude has remained virtually undiminished over the past 20 years despite considerable advances in understanding most of the key contributing elements. Recent wo ...

AMER GEOPHYSICAL UNION2023

MoMuCAMS: A new modular platform for boundary layer aerosol and trace gas vertical measurements in extreme environments

Julia Schmale, Andrea Baccarini, Roman Pohorsky

The Modular Multiplatform Compatible Air Measurement System (MoMuCAMS) is a newly developed in situ aerosol and trace gas measurement payload for lower atmospheric vertical profiling in extreme environments. MoMuCAMS is a multiplatform compatible system, p ...

2023

A full year of aerosol size distribution data from the central Arctic under an extreme positive Arctic Oscillation: insights from the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition

Julia Schmale, Benjamin Jérémy Laurent Heutte, Jakob Boyd Pernov, Ivo Fabio Beck, Hélène Paule Angot, Lubna Dada, Federico Bianchi

The Arctic environment is rapidly changing due to accelerated warming in the region. The warming trend is driving a decline in sea ice extent, which thereby enhances feedback loops in the surface energy budget in the Arctic. Arctic aerosols play an importa ...

Copernicus Publications2023

Measurements of aerosol microphysical and chemical properties in the central Arctic atmosphere during MOSAiC

Julia Schmale, Benjamin Jérémy Laurent Heutte, Nora Bergner, Ivo Fabio Beck, Hélène Paule Angot, Lubna Dada

The Arctic environment is transforming rapidly due to climate change. Aerosols’ abundance and physicochemical characteristics play a crucial, yet uncertain, role in these changes due to their influence on the surface energy budget through direct interactio ...

2023

Pan-Arctic seasonal cycles and long-term trends of aerosol properties from 10 observatories

Julia Schmale, Jakob Boyd Pernov

Even though the Arctic is remote, aerosol properties observed there are strongly influenced by anthropogenic emissions from outside the Arctic. This is particularly true for the so-called Arctic haze season (January through April). In summer (June through ...

Copernicus Publications2022

Elucidating the present-day chemical composition, seasonality and source regions of climate-relevant aerosols across the Arctic land surface

Julia Schmale, Imad El Haddad

The Arctic is warming two to three times faster than the global average, and the role of aerosols is not well constrained. Aerosol number concentrations can be very low in remote environments, rendering local cloud radiative properties highly sensitive to ...

IOP Publishing Ltd2022

Observed coupling between air mass history, secondary growth of nucleation mode particles and aerosol pollution levels in Beijing

Lubna Dada, Yu Fu, François Bianchi, Jingjing Jiang

Atmospheric aerosols have significant effects on the climate and on human health. New particle formation (NPF) is globally an important source of aerosols but its relevance especially towards aerosol mass loadings in highly polluted regions is still contro ...

2022

Numerical investigation of the effect of cohesion and ground friction on snow avalanches flow regimes

Johan Alexandre Philippe Gaume, Betty Sovilla

With ongoing global warming, snow avalanche dynamics may change as snow cohesion and friction strongly depend on temperature. In the field, a diversity of avalanche flow regimes has been reported including fast, sheared flows and slow plugs. While the sign ...

PUBLIC LIBRARY SCIENCE2022

Equal abundance of summertime natural and wintertime anthropogenic Arctic organic aerosols

Julia Schmale, Imad El Haddad, Houssni Lamkaddam, Pragati Rai

Aerosols play an important yet uncertain role in modulating the radiation balance of the sensitive Arctic atmosphere. Organic aerosol is one of the most abundant, yet least understood, fractions of the Arctic aerosol mass. Here we use data from eight obser ...

2022

Using stratospheric aerosol injection to alleviate global warming: when?

Marie-Valentine Renée Agnès Florin

Stratospheric aerosol injection (SAI), a type of solar radiation modification (SRM), has the potential to reduce global warming caused by excessive greenhouse gases in the atmosphere. However, there is currently widespread opposition to it, because deployi ...

EPFL International Risk Governance Center (IRGC).2021

Low‐Volatility Vapors and New Particle Formation Over the Southern Ocean During the Antarctic Circumnavigation Expedition

Julia Schmale, Andrea Baccarini, Robin Lewis Modini

During summer, the Southern Ocean is largely unaffected by anthropogenic emissions, which makes this region an ideal place to investigate marine natural aerosol sources and processes. A better understanding of natural aerosol is key to constrain the preind ...

2021

Dynamic spatiotemporal patterns of brain connectivity reorganize across development

Alessandra Griffa, Patric Hagmann, Marie Schaer, Emeline Mullier

Late human development is characterized by the maturation of high-level functional processes, which rely on reshaping of white matter connections, as well as synaptic density. However, the relationship between the whole-brain dynamics and the underlying wh ...

MIT PRESS2020

Source apportionment of atmospheric P using the Positive Matrix Factorization (PMF) model

Athanasios Nenes, Kalliopi Violaki, Christos Panagiotopoulos

The PMF receptor model was applied to a combined dataset using specific markers such as phospholipids and sugars together with other metals (e.g. Al, Pb, V) and ions (e.g. K+, Ca2+, SO42-, NO3-) as tracers of main aerosol sources in order to characterize t ...

2020

Drivers of cloud droplet number variability in the summertime in the southeastern United States

Athanasios Nenes, André Welti

Here we analyze regional-scale data collected on board the NOAA WP-3D aircraft during the 2013 Southeast Nexus (SENEX) campaign to study the aerosol-cloud droplet link and quantify the sensitivity of droplet number to aerosol number, chemical composition, ...

Copernicus GmbH2020

Size distribution of aerosol particles between 2.5 and 920 nm measured during the Arctic Ocean 2018 expedition

Julia Schmale, Andrea Baccarini

The aerosol size distribution was obtained combining measurements from a neutral and air ion spectrometer (NAIS) with a differential mobility particle sizer (DMPS). Merging particle size distribution (PSD) measurements from different instruments allows to ...

2020

Conversion of vine shoots into bioethanol and chemicals: Prospective LCA of biorefinery concept

Edgard Gnansounou, Elia Mercedes Ruiz Pachon, Prasad Vithalrao Mandade

Vine shoots are the viticulture residues generated in high quantities after the grapevine pruning. They are lignocellulosic material poorly exploited as feedstock. These wastes are often dumped in the agriculture fields or burnt. Due to their availability ...

Elsevier2020

Size distribution of interstitial and total particles between 18 and 660 nm collected during the Arctic Ocean 2018 expedition

Julia Schmale, Andrea Baccarini

The aerosol size distribution was measured with a custom made scanning mobility particle sizer (SMPS), range 18⁠ – ⁠660 nm. Aerosols are important for a variety of reasons, one of the most prominent is that a sub-set of the aerosol population can act as cl ...

2020

Three-dimensional radiative transfer effects on airborne and ground-based trace gas remote sensing

Alexis Berne, Dominik Brunner, Thomas Wagner

Air mass factors (AMFs) are used in passive trace gas remote sensing for converting slant column densities (SCDs) to vertical column densities (VCDs). AMFs are traditionally computed with 1D radiative transfer models assuming horizontally homogeneous condi ...

2020