Publications associées à Gaz de couche

Deep learning-based recommendation system for metal-organic frameworks (MOFs)

Berend Smit, Xiaoqi Zhang, Kevin Maik Jablonka

This work presents a recommendation system for metal-organic frameworks (MOFs) inspired by online content platforms. By leveraging the unsupervised Doc2Vec model trained on document-structured intrinsic MOF characteristics, the model embeds MOFs into a hig ...

Royal Soc Chemistry2024

Design and assessment of an evaporating water-cooled methanation reactor for a SOE-based power-to-methane system

Philippe Aubin

The transition towards clean renewable energy sources, where wind and solar are prone to variation, requires adequate energy storage. Power-to-methane (PtM) systems can be part of the solution. Specifically, solid-oxide-electrolyser (SOE) based PtM systems ...

EPFL2024

Comparative Exergy and Economic Assessment of Fossil and Biomass-Based Routes for Ammonia Production

François Maréchal, Daniel Alexander Florez Orrego

Due to the increasing concerns about the marked dependence on fossil resources and their intrinsic economic uncertainty, as well as motivated by more stringent environmental regulations, the pursuit of alternative energy resources for the synthetic fertili ...

Silesian University of Technology2023

Reactivation of variably sealed joints and permeability enhancement in geothermal reservoir rocks

Alexandra Roma Larisa Kushnir, Michael Heap

Hydraulic stimulation of enhanced deep geothermal reservoirs commonly targets pre-existing joint networks with the goal of increasing reservoir permeability. Here, we study the permeability and strength of joint-free and jointed Buntsandstein sandstones fr ...

2023

Emission reduction by targeted transient operations in three-way catalysts for heavy-duty natural gas applications

Moyu Wang

To curb the severe effects of climate change, our society needs to radically reduce its CO2 footprint. For the heavy-duty sector, where electrification is difficult, alternative fuels can be the solution. Methane-fueled engines have lower energy-specific C ...

EPFL2022

Investigation on the Role of Pd, Pt, Rh in Methane Abatement for Heavy Duty Applications

Oliver Kröcher, Davide Ferri, Moyu Wang

Methane abatement remains a challenge in aftertreatment systems of natural gas engines, currently under discussion in combination with synthetic methane. In this study, Pt/Rh and Pd/Rh-based three-way catalysts are investigated under various transient cond ...

MDPI2022

Swelling and shrinkage of partially saturated gas shales: from laboratory tests to an effective stress framework

Jinwoo Kim

Gas shale swelling during hydraulic stimulation is one of the major challenges in unconventional gas development. It is hypothesized that the large volumetric strain upon water imbibition is a consequence of dramatic changes in capillary pressure and disjo ...

EPFL2022

Flexible application of biogas upgrading membranes for hydrogen recycle in power-to-methane processes

Oliver Kröcher, Andreas Gantenbein

Direct methanation of biogas converts the CO2 in raw-biogas to methane, enabling higher methane yield and an elelctricity storage option via Power-to-Gas. As the thermodynamic equilibrium limits the methane yield, unreacted hydrogen has to be removed and r ...

Elsevier2021

Gold-in-copper at low *CO coverage enables efficient electromethanation of CO2

Michael Graetzel, Dan Ren, Yang Li, Jun Li, Yongfeng Xie, Xiaoyan Wang, Yiping Wang, Ziyun Wang, Pengfei Ou, Yi Xu

The renewable-electricity-powered CO2 electroreduction reaction provides a promising means to store intermittent renewable energy in the form of valuable chemicals and dispatchable fuels. Renewable methane produced using CO2 electroreduction attracts inter ...

Nature Research2021

Reaction pathways of methane abatement in Pd-Rh three-way catalyst in heavy duty applications: A combined approach based on exhaust analysis, model gas reactor and DRIFTS measurements

Oliver Kröcher, Davide Ferri, Moyu Wang

Methane abatement pathways in Pd/Rh three-way catalysts have been investigated in three scales ranging from a vehicle application size catalyst, a model gas reactor and the catalyst in powder form. A special test rig was designed for the investigation of v ...

ELSEVIER SCIENCE SA2021

Microbial-induced carbonate precipitation applicability with the methane hydrate-bearing layer microbe

Alexandra Clarà Saracho

Production of methane gas from the methane-hydrate-bearing layer below the deep-ocean floor is expected to be crucial in the future of energy resources worldwide. During the methane gas-production phase from the methane hydrate with the depressurisation me ...

ELSEVIER SCI LTD2020

Direct conversion of plastic materials into methane and liquid fuels

Paul Joseph Dyson, Felix Daniel Bobbink, Antoine Philippe Van Muyden, Wei-Tse Lee

The invention relates to a method for direct conversion of plastic materials into methane and/or liquid fuel and use of ruthenium-modified zeolite to catalyse this conversion. ...

2020

Lateral variations and vertical structure of the microbial methane cycle in the sediment of Lake Onego (Russia)

Natacha Tofield-Pasche, Nathalie Dubois

The significance of methane production by lakes to the global production of greenhouse gas is well acknowledged while underlying processes sustaining the lacustrine methane budget remain largely unknown. We coupled biogeochemical data to functional and phy ...

2019

Exploring the Sources of Unexpected High Methane Concentrations and Fluxes From Alpine Headwater Streams

Amber Joy Ulseth, Sabine Flury McGinnis

The dynamics of methane generation and evasion from well-oxygenated, oligotrophic streams have been traditionally neglected. We estimated evasion of methane and assessed its sources and production pathways using a stable isotope approach in 16 oxygen-rich ...

AMER GEOPHYSICAL UNION2019

Efficient Base-Metal NiMn/TiO2 Catalyst for CO2 Methanation

Andreas Züttel, Emanuele Moioli, Wei Chen

Energy storage solutions are a vital component of the global transition toward renewable energy sources. The power-to-gas (PtG) concept, which stores surplus renewable energy in the form of methane, has therefore become increasingly relevant in recent year ...

2019

Elastic behavior of partially saturated gas shales during unloading - reloading cycles in uniaxial compression

Lyesse Laloui, Alessio Ferrari, Alberto Minardi

Elastic properties of gas shales are of utmost importance for the exploitation of shale gas reservoirs. Static elastic properties are usually measured by performing unloading-reloading cycles in uniaxial or triaxial compressive tests. The response of gas s ...

2018

Guest dynamics in methane hydrates and hydrogen hydrates under high pressure

Umbertoluca Ranieri

Hydrates of gas are non-stoichiometric inclusion compounds constituted of water and gas. Therein, the water molecules are hydrogen-bonded and form three-dimensional crystalline networks incorporating different kinds of polar or nonpolar guest gas molecules ...

EPFL2018

Impact of the strength and spatial distribution of adsorption sites on methane deliverable capacity in nanoporous materials

Berend Smit, Cory Matthew Simon

The methane deliverable capacity of adsorbent materials is a critical performance metric that will determine the viability of using adsorbed natural gas (ANG) technology in vehicular applications. ARPA-E recently set a target deliverable capacity of 315 cc ...

Elsevier2017

Full-scale evaluation of methane production under oxic conditions in a mesotrophic lake

Sabine Flury McGinnis

Oxic lake surface waters are frequently oversaturated with methane (CH4). The contribution to the global CH4 cycle is significant, thus leading to an increasing number of studies and stimulating debates. Here we show, using a mass balance, on a temperate, ...

Nature Publishing Group2017

Material constraints related to storage of future European renewable electricity surpluses with CO2 methanation

Vincent Moreau, Suren Erkman

The main challenges associated with a growing production of renewable electricity are intermittency and dispersion. Intermittency generates spikes in production, which need to be curtailed when exceeding consumption. Dispersion means electricity has to be ...

Elsevier2016