Publications de Karla Banjac | EPFL Graph Search

Operando Nanoscale Characterization Reveals Fe Doping of Ni Oxide Enhances Oxygen Evolution Reaction via Fragmentation and Formation of Dual Active Sites

Magalí Alejandra Lingenfelder, Xile Hu, Karla Banjac, Seunghwa Lee, Yunchang Liang, Victor Carle Adrien Boureau

Efficient catalytic water splitting demands advanced catalysts to improve the slow kinetics of the oxygen evolution reaction (OER). Earth-abundant transition metal oxides show promising OER activity in alkaline media. However, most experimental information ...

2025

Enhancement of electrocatalytic oxygen evolution by chiral molecular functionalization of hybrid 2D electrodes

Magalí Alejandra Lingenfelder, Xile Hu, Karla Banjac, Seunghwa Lee, Yunchang Liang

While solar-to-fuel catalysis requires the careful transfer of electrons, there are still challenges understanding how electron spin contributes to reactivity. Here, authors employ chiral fused thiadiazole-helicenes to control spin polarization in oxygen e ...

Nature Portfolio2022

In situ nanoscale studies of copper-based catalysts for carbon dioxide electroreduction

Karla Banjac

The urgency of climate change demands the simultaneous removal of carbon dioxide from the atmosphere and the transition to renewable energy sources. This aim is realizable through electrochemical reduction of carbon dioxide (CO2RR), which is a promising ro ...

EPFL2021

Structural Order of the Molecular Adlayer Impacts the Stability of Nanoparticle-on-Mirror Plasmonic Cavities

Magalí Alejandra Lingenfelder, Christophe Marcel Georges Galland, Fernando Pablo Cometto, Karla Banjac, Aqeel Ahmed, Sachin Suresh Verlekar

Immense field enhancement and nanoscale confinement of light are possible within nanoparticle-on-mirror (NPoM) plasmonic resonators, which enable novel optically activated physical and chemical phenomena and render these nanocavities greatly sensitive to m ...

AMER CHEMICAL SOC2021

Intrinsic luminescence blinking from plasmonic nanojunctions

Magalí Alejandra Lingenfelder, Christophe Marcel Georges Galland, Tobias Kippenberg, Philippe Andreas Rölli, Giulia Tagliabue, Karla Banjac, Aqeel Ahmed, Wen Chen, Sachin Suresh Verlekar

Plasmonic nanojunctions, consisting of adjacent metal structures with nanometre gaps, can support localised plasmon resonances that boost light matter interactions and concentrate electromagnetic fields at the nanoscale. In this regime, the optical respons ...

Nature Research2021

Super-resolved Optical Mapping of Reactive Sulfur-Vacancies in Two-Dimensional Transition Metal Dichalcogenides

Andras Kis, Aleksandra Radenovic, Magalí Alejandra Lingenfelder, Jean Camille Benjamin Comtet, Martina Lihter, Yanfei Zhao, Michal Daniel Macha, Karla Banjac, Jing Zhang, Zhenyu Wang, Miao Zhang, Tzu-Heng Chen

Transition metal dichalcogenides (TMDs) represent a class of semiconducting two-dimensional (2D) materials with exciting properties. In particular, defects in 2D-TMDs and their molecular interactions with the environment can crucially affect their physical ...

AMER CHEMICAL SOC2021

Emergence of Potential-Controlled Cu-Nanocuboids and Graphene-Covered Cu-Nanocuboids under Operando CO2 Electroreduction

Magalí Alejandra Lingenfelder, Fernando Pablo Cometto, Karla Banjac, Thanh Hai Phan

The electroreduction of CO2 (CO2RR) is a promising strategy toward sustainable fuels. Cu is the only Earth-abundant and pure metal capable of catalyzing CO2-to-hydrocarbons conversion with significant Faradaic efficiencies; yet, its dynamic structure under ...

AMER CHEMICAL SOC2021

Oxygen Isotope Labeling Experiments Reveal Different Reaction Sites for the Oxygen Evolution Reaction on Nickel and Nickel Iron Oxides

Magalí Alejandra Lingenfelder, Xile Hu, Karla Banjac, Seunghwa Lee

Nickel iron oxide is considered a benchmark nonprecious catalyst for the oxygen evolution reaction (OER). However, the nature of the active site in nickel iron oxide is heavily debated. Here we report direct spectroscopic evidence for the different active ...

Wiley-VCH Verlag GmbH2019