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Felix Thomas Eickemeyer

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Publications associées (57)

Surface Passivation of FAPbI3-Rich Perovskite with Cesium Iodide Outperforms Bulk Incorporation

Michael Graetzel, Jacques-Edouard Moser, Shaik Mohammed Zakeeruddin, Mounir Driss Mensi, Jun Ho Yum, Kevin Sivula, Thomas Paul Baumeler, Essa Awadh R Alharbi, Brian Irving Carlsen, Jing Gao, George Cameron Fish, Felix Thomas Eickemeyer, Lukas Pfeifer, Georgios Kakavelakis

Metal halide perovskites (MHPs) have shown an incredible increase in efficiency, reaching as high as 25.7%, which now competes with traditional photovoltaic technologies. Herein, we excluded CsX and RbX (X = I–, Br–, Cl–), the most commonly used cations to ...

2023

Bifunctional hole-shuttle molecule for improved interfacial energy level alignment and defect passivation in perovskite solar cells

Michael Graetzel, Shaik Mohammed Zakeeruddin, Jun Ho Yum, Kevin Sivula, Dan Ren, Jing Gao, Meng Xia, Felix Thomas Eickemeyer, Zhongjin Shen

Interface engineering in perovskite solar cells is key to high performance. Now, You et al. design an interlayer that both passivates defects and improves the energy level alignment between the perovskite and hole transport material. ...

NATURE PORTFOLIO2023

Cooperative passivation of perovskite solar cells by alkyldimethylammonium halide amphiphiles

Michael Graetzel, Shaik Mohammed Zakeeruddin, Ursula Röthlisberger, Ulf Anders Hagfeldt, Thomas Paul Baumeler, David Lyndon Emsley, Essa Awadh R Alharbi, Mathias Dankl, Aditya Mishra, Felix Thomas Eickemeyer, Michael Allan Hope, Anurag Krishna, Olivier Ouellette, Lukas Pfeifer, Nikolaos Lempesis, Georgios Kakavelakis

2023

Indoor Self-Powered Perovskite Optoelectronics with Ultraflexible Monochromatic Light Source

Felix Thomas Eickemeyer, Tommaso Marcato, Hiroaki Jinno, Lukas Pfeifer

Self-powered skin optoelectronics fabricated on ultrathin polymer films is emerging as one of the most promising components for the next-generation Internet of Things (IoT) technology. However, a longstanding challenge is the device underperformance owing ...

Wiley-V C H Verlag Gmbh2023

Buried Interface Engineering Enables Efficient and 1,960-hour Isos-L-2i Stable Inverted Perovskite Solar Cells

Michael Graetzel, Shaik Mohammed Zakeeruddin, Ursula Röthlisberger, Xiong Li, Mathias Dankl, Felix Thomas Eickemeyer, Nikolaos Lempesis, Mingyang Wei, Virginia Carnevali, Lorenzo Agosta, Lin Li

High-performance perovskite solar cells (PSCs) typically require interfacial passivation, yet this is challenging for the buried interface, owing to the dissolution of passivation agents during the deposition of perovskites. Here, we overcome this limitati ...

Zenodo2023

Stabilization of FAPbI(3) with Multifunctional Alkali-Functionalized Polymer

Michael Graetzel, Shaik Mohammed Zakeeruddin, Jing Gao, Masaud Hassan S Almalki, Felix Thomas Eickemeyer, Hong Zhang, Anurag Krishna

The defects located at the interfaces and grain boundaries (GBs) of perovskite films are detrimental to the photovoltaic performance and stability of perovskite solar cells. Manipulating the perovskite crystallization process and tailoring the interfaces w ...

Wiley-V C H Verlag Gmbh2023

Molecular engineering of low-cost, efficient, and stable photosensitizers for dye-sensitized solar cells

Michael Graetzel, Shaik Mohammed Zakeeruddin, Marina Freitag, Jing Gao, Felix Thomas Eickemeyer, Zhongjin Shen, Lukas Pfeifer

The cost, stability, and photovoltaic performance of photosensi-tizers play a key role in the commercialization of dye-sensitized solar cells (DSCs). Herein, three novel sensitizers termed ZS10, ZS11, and ZS12 are described based on the simple chemical str ...

Cell Press2023

Interfacial Modulation through Mixed-Dimensional Heterostructures for Efficient and Hole Conductor-Free Perovskite Solar Cells

Michael Graetzel, Shaik Mohammed Zakeeruddin, Anwar Qasem M Alanazi, Jovana Milic, Felix Thomas Eickemeyer, Hong Zhang, Laura Piveteau

Perovskite solar cells have led the new surge of solar energy research. However, their instability is a pressing issue mostly attributed to the perovskite interface with charge-selective transport layers. In this work, diethylammonium iodide (DEAI) surface ...

Wiley-V C H Verlag Gmbh2023

Nanocrystalline Flash Annealed Nickel Oxide for Large Area Perovskite Solar Cells

Michael Graetzel, Jovana Milic, Felix Thomas Eickemeyer

The industrialization of perovskite solar cells requires adequate materials and processes to make them economically viable and environmentally sustainable. Despite promising results in terms of power conversion efficiency and operational stability, several ...

WILEY2023

Engineering ligand reactivity enables high-temperature operation of stable perovskite solar cells

Michael Graetzel, Shaik Mohammed Zakeeruddin, Thi Thu Trang Pham, Zaiwei Wang, Felix Thomas Eickemeyer, Jian Xu, Mingyang Wei, Cheng Liu

Perovskite solar cells (PSCs) consisting of interfacial two- and three-dimensional heterostructures that incorporate ammonium ligand intercalation have enabled rapid progress toward the goal of uniting performance with stability. However, as the field cont ...

American Association for the Advancement of Science2023

Radical polymeric p-doping and grain modulation for stable, efficient perovskite solar modules

Michael Graetzel, Shaik Mohammed Zakeeruddin, Yuhang Liu, Brian Irving Carlsen, Felix Thomas Eickemeyer

High-quality perovskite light harvesters and robust organic hole extraction layers are essential for achieving high-performing perovskite solar cells (PSCs). We introduce a phosphonic acid???functionalized fullerene derivative in mixed-cation perovskites a ...

American Association for the Advancement of Science2023

Mitigating the Heterointerface Driven Instability in Perovskite Photovoltaics

Michael Graetzel, Shaik Mohammed Zakeeruddin, Ursula Röthlisberger, Ulf Anders Hagfeldt, Essa Awadh R Alharbi, Mathias Dankl, Felix Thomas Eickemeyer, Hong Zhang, Anurag Krishna

Metal halide perovskites have thepotential to revolutionizethefield of photovoltaics, though limited stability has impeded commercialexploitation. The soft heterointerface between the perovskite andcharge-transporting layer is one of the major bottlenecks ...

AMER CHEMICAL SOC2023

Hydroxamic acid pre-adsorption raises the efficiency of cosensitized solar cells

Michael Graetzel, Shaik Mohammed Zakeeruddin, Nikolaos Vlachopoulos, Ulf Anders Hagfeldt, Yiming Cao, Felix Thomas Eickemeyer, Yameng Ren, Dan Zhang, Jiajia Suo

Dye-sensitized solar cells (DSCs) convert light into electricity by using photosensitizers adsorbed on the surface of nanocrystalline mesoporous titanium dioxide (TiO2) films along with electrolytes or solid charge-transport materials(1-3). They possess ma ...

NATURE PORTFOLIO2023

High-Work-Function 2D Perovskites as Passivation Agents in Perovskite Solar Cells

Michael Graetzel, Mohammad Khaja Nazeeruddin, Paul Joseph Dyson, Ulf Anders Hagfeldt, Antoine Philippe Van Muyden, Farzaneh Fadaei Tirani, Erfan Shirzadi, Hiroyuki Kanda, Brian Irving Carlsen, Fatemeh Ansari, Felix Thomas Eickemeyer, Olivier Ouellette, Hiroaki Jinno

Various approaches have been employed to passivate the defects in perovskite films used in perovskite solar cells (PSCs). However, the passivation mechanism is often unclear at a molecular level, and the reason for enhanced PSC performance often remains el ...

Amer Chemical Soc2023

A Molecularly Tailored Photosensitizer with an Efficiency of 13.2% for Dye-Sensitized Solar Cells

Michael Graetzel, Shaik Mohammed Zakeeruddin, Felix Thomas Eickemeyer, Zhongjin Shen, Naura Fakhira Antariksa

Photosensitizers yielding superior photocurrents are crucial for copper-electrolyte-based highly efficient dye-sensitized solar cells (DSCs). Herein, two molecularly tailored organic sensitizers are presented, coded ZS4 and ZS5, through judiciously employi ...

Wiley-V C H Verlag Gmbh2023

Thermally controlled growth of photoactive FAPbI(3) films for highly stable perovskite solar cells

Michael Graetzel, Shaik Mohammed Zakeeruddin, Cyril Cayron, Sandy Sanchez Alonso, Pascal Alexander Schouwink, Felix Thomas Eickemeyer

We employ flash infrared annealing to investigate the phase transition of formamidinium lead triiodide (FAPbI(3)) thin films for their solar cell applications. Measuring the enthalpy changes of the FAPbI(3) composition at different heating rates allows us ...

ROYAL SOC CHEMISTRY2022

Conformal quantum dot-SnO2 layers as electron transporters for efficient perovskite solar cells

Michael Graetzel, Shaik Mohammed Zakeeruddin, Yuhang Liu, Haizhou Lu, Felix Thomas Eickemeyer, Jaeki Jeong

Improvements to perovskite solar cells (PSCs) have focused on increasing their power conversion efficiency (PCE) and operational stability and maintaining high performance upon scale-up to module sizes. We report that replacing the commonly used mesoporous ...

American Association for the Advancement of Science2022

Enabling full-scale grain boundary mitigation in polycrystalline perovskite solids

Michael Graetzel, Shaik Mohammed Zakeeruddin, Ulf Anders Hagfeldt, Jingshan Luo, Lichen Zhao, Yuhang Liu, Felix Thomas Eickemeyer

There exists a considerable density of interaggregate grain boundaries (GBs) and intra-aggregate GBs in polycrystalline perovskites. Mitigation of intra- aggregate GBs is equally notable to that of interaggregate GBs as intra-aggregate GBs can also cause d ...

AMER ASSOC ADVANCEMENT SCIENCE2022

Efficient and Stable Large Bandgap MAPbBr(3) Perovskite Solar Cell Attaining an Open Circuit Voltage of 1.65 V

Michael Graetzel, Shaik Mohammed Zakeeruddin, Thomas Paul Baumeler, David Lyndon Emsley, Linfeng Pan, Anwar Qasem M Alanazi, Yuhang Liu, Jing Gao, Felix Thomas Eickemeyer, Hongwei Zhu, Michael Allan Hope, Olivier Ouellette

We report on the preparation of MAPbBr(3) perovskite films of high electronic quality by applying a methylamine (MA) vapor treatment and mitigating surface defects using the amphiphilic molecular passivator, neopentylammonium chloride (NPACl). We find that ...

2022

Methylammonium Triiodide for Defect Engineering of High-Efficiency Perovskite Solar Cells

Michael Graetzel, Jacques-Edouard Moser, Shaik Mohammed Zakeeruddin, Mounir Driss Mensi, Ursula Röthlisberger, Ulf Anders Hagfeldt, Thomas Paul Baumeler, Linfeng Pan, Paramvir Ahlawat, Claudia Esther Avalos, Essa Awadh R Alharbi, Pascal Alexander Schouwink, George Cameron Fish, Mathias Dankl, Bowen Yang, Felix Thomas Eickemeyer, Viktor Skorjanc, Anurag Krishna, Olivier Ouellette, Elsa John, Lukas Pfeifer

The defects present in metal halide perovskite are deleterious to both the performance and stability of photovoltaic devices. Consequently, there is an intense focus on developing defect mitigation strategies. Herein we report a facile strategy that employ ...

2021

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