Publications associées à Unusual Rydberg System Consisting of a Positively Charged Helium Nanodroplet with an Orbiting Electron

Magnetism of Single Surface Adsorbed Atoms Studied with Radio-Frequency STM

This thesis investigates the magnetic properties of single atoms and molecules adsorbed on thin magnesium oxide decoupling layers, grown on a silver single crystal. To address these systems experimentally, we use a low temperature scanning tunneling micros ...

EPFL2024

Valence Orbitals Driving the Spin Dynamics in a Rare-Earth Single-Atom Magnet

Harald Brune, François Patthey, Stefano Rusponi, Marina Pivetta, Dante Philippe Sblendorio, Alberto Curcella

We combine spin-polarized scanning tunneling microscopy with quantum master equation analysis to investigate the spin dynamics of the single atom magnet Dy on graphene/Ir(111). By performing reading and writing experiments, we show that the strongly spin p ...

AMER PHYSICAL SOC2023

Validation of 2D T e and n e measurements made with Helium imaging spectroscopy in the volume of the TCV divertor

Patrick Blanchard, Basil Duval, Holger Reimerdes, Christian Gabriel Theiler, Hugo De Oliveira, Cedric Kar-Wai Tsui, Nicola Offeddu, Filippo Bagnato, Lorenzo Martinelli, Sophie Danielle Angelica Gorno, Claudia Colandrea, Dmytry Mykytchuk, Artur Perek

Multi-spectral imaging of helium atomic emission (HeMSI) has been used to create 2D poloidal maps of T-e and ne in TCV's divertor. To achieve these measurements, TCV's MANTIS multispectral cameras (Perek et al 2019 Rev. Sci. Instrum. 90 123514) simultaneou ...

IOP Publishing Ltd2023

The role of plasma-atom and molecule interactions on power & particle balance during detachment on the MAST Upgrade Super-X divertor

Christian Gabriel Theiler, Kevin Henricus Annemarie Verhaegh

This paper shows first quantitative analysis of the detachment processes in the MAST Upgrade Super-X divertor (SXD). We identify an unprecedented impact of plasma-molecular interactions involving molecular ions (likely D2+ ), resulting in strong ion sinks ...

IOP Publishing Ltd2023

On Quantum Secure Compressing Pseudorandom Functions

Ritam Bhaumik

In this paper we characterize all 2n-bit-to-n-bit Pseudorandom Functions (PRFs) constructed with the minimum number of calls to n-bit-to-n-bit PRFs and arbitrary number of linear functions. First, we show that all two-round constructions are either classic ...

2023

Strain Gradients and Magnetoresistance in Microstructured 3D Topological Semi-metals

Jonas De Jesus Diaz Gomez

Three-dimensional topological semimetals have emerged as strong candidates to probe new fundamental physical phenomena that could be exploited to develop next generation electronics. However, many aspects of their electronic properties remain unclear. Thi ...

EPFL2023

In situ work function measurements of W, WO3 nanostructured surfaces

Francisco Sanchez

Surface nanostructuring enables the fabrication of materials with highly desirable properties. Nanostructured tungsten surfaces have potential applications in solar water splitting. Exposing a polished tungsten surface to helium plasma induces various surf ...

ELSEVIER SCIENCE SA2022

Spectral properties of extended systems from Koopmans-compliant functionals

Riccardo De Gennaro

Electronic-structure simulations have been impacting the study of materials properties thanks to the simplicity of density-functional theory, a method that gives access to the ground state of the system. Although very important, ground-state properties rep ...

EPFL2022

Unified theory of atom-centered representations and message-passing machine-learning schemes

Michele Ceriotti, Jigyasa Nigam, Guillaume André Jean Fraux, Sergey Pozdnyakov

Data-driven schemes that associate molecular and crystal structures with their microscopic properties share the need for a concise, effective description of the arrangement of their atomic constituents. Many types of models rely on descriptions of atom-cen ...

AIP Publishing2022

Cavity Quantum Electrodynamics with strongly correlated fermions

Kevin Etienne Robert Roux

This thesis presents the first cavity quantum electrodynamics experiments performed with a degenerate gas of

^6

Li with strong atom-atom interactions. The first part of this manuscript describes the design and the building of the apparatus that has been e ...

EPFL2022

Long Spin Lifetime in Rare-Earth Single-Atom Magnets at Surfaces

Boris Sorokin

Further miniaturisation of magnetic storage devices requires an advent of new types of magnets, since classical ferromagnetic materials show lack of remanence at nano- and subnanoscale. A single atom can represent the smallest possible bit of information. ...

EPFL2022

Quantum Circuits for the Preparation of Spin Eigenfunctions on Quantum Computers

Alessandro Carbone

The application of quantum algorithms to the study of many-particle quantum systems requires the ability to prepare wave functions that are relevant in the behavior of the system under study. Hamiltonian symmetries are important instruments used to classif ...

MDPI2022

Mapping Orbital-Resolved Magnetism in Single Lanthanide Atoms

Harald Brune, Stefano Rusponi, Marina Pivetta, Fabio Donati, Aparajita Singha

Single lanthanide atoms and molecules are promising candidates for atomic data storage and quantum logic due to the long lifetime of their magnetic quantum states. Accessing and controlling these states through electrical transport requires precise knowled ...

AMER CHEMICAL SOC2021

Hunting for tetraquarks in ultraperipheral heavy ion collisions

Claudio Andrea Manzari, Angelo Esposito

Ultraperipheral heavy ion collisions constitute an ideal setup to look for exotic hadrons because of their low event multiplicity and the possibility of an efficient background rejection. We propose to look for fourquark states produced by photon-photon fu ...

American Physical Society2021

Observation of a New Excited Beauty Strange Baryon Decaying to Xi(-)(b)pi(+)pi(-)

Rakesh Chawla, Arvind Shah, Andrea Rizzi, Matthias Finger, Bandeep Singh, Federica Legger, Thomas Berger, Jian Zhao, João Miguel das Neves Duarte, Tagir Aushev, Hua Zhang, Alexis Kalogeropoulos, Chao Wang, Yixing Chen, Tian Cheng, Ioannis Papadopoulos, Marco Pisano, Valérie Scheurer, Meng Xiao, Wei Sun, Maren Tabea Meinhard, Qian Wang, Michele Bianco, Doohyun Kim, Varun Sharma, Jessica Prisciandaro, Joao Varela, Francesco Fiori, Sourav Sen, Ashish Sharma, Seungkyu Ha, David Vannerom, Csaba Hajdu, Sanjeev Kumar, Sebastiana Gianì, Kun Shi, Abhisek Datta, Guido Andreassi, Miao Hu, Siyuan Wang, Peter Hansen, Muhammad Waqas, , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , ,

Competitive Dehydrogenation and Backbone Fragmentation of Superhydrogenated PAHs: A Laboratory Study

Robert Richter, Eduardo Carrascosa Casado

Superhydrogenated polycyclic aromatic hydrocarbons (PAHs) have been suggested to catalyze the formation of H-2 in certain regions of space, but it remains unclear under which circumstances this mechanism is viable given the reduced carbon backbone stabilit ...

2021

Laser photo-detachment combined with Langmuir probe in magnetized electronegative plasma: how the probe size affects the plasma dynamic?

Ivo Furno, Riccardo Agnello

Laser photo-detachment combined with a Langmuir probe (LP) is used to diagnose negative ion properties in electronegative plasmas. The technique relies on the combined use of a laser pulse and an LP. The laser pulse converts negative ions into electron-ato ...

2021

Weakness of Correlation Effect Manifestation in BaNi2As2: An ARPES and LDA plus DMFT Study

Daniil Yevtushynsky, Timur Kim

The electronic spectral function of BaNi2As2 is investigated using both angle-resolved photoemission spectroscopy (ARPES) and a combined computational scheme of local density approximation and dynamical mean-field theory (LDA + DMFT). In contrast to the we ...

AMER CHEMICAL SOC2021

Charging and ion ejection dynamics of large helium nanodroplets exposed to intense femtosecond soft X-ray pulses

Daniela Rupp, Camila Bacellar Cases Da Silveira, Christoph Bostedt

Ion ejection from charged helium nanodroplets exposed to intense femtosecond soft X-ray pulses is studied by single-pulse ion time-of-flight (TOF) spectroscopy in coincidence with small-angle X-ray scattering. Scattering images encode the droplet size and ...

SPRINGER HEIDELBERG2021

Using collective knowledge to assign oxidation states of metal cations in metal-organic frameworks

Seyedmohamad Moosavi, Berend Smit, Daniele Ongari, Kevin Maik Jablonka

Knowledge of the oxidation state of metal centres in compounds and materials helps in the understanding of their chemical bonding and properties. Chemists have developed theories to predict oxidation states based on electron-counting rules, but these can f ...

NATURE RESEARCH2021