Publications associées à Relationship between high daily erythemal UV doses, total ozone, surface albedo and cloudiness: An analysis of 30 years of data from Switzerland and Austria

Nanocluster Aerosols from Ozone-Human Chemistry Are Dominated by Squalene-Ozone Reactions

Dusan Licina, Shen Yang

Nanocluster aerosols (NCAs,

Amer Chemical Soc2024

Nanocluster aerosol formation via ozone chemistry on worn clothing: Influence of environmental parameters

Dusan Licina, Shen Yang

Nanocluster aerosols (NCA, particles

Pergamon-Elsevier Science Ltd2024

Influence of Ventilation on Formation and Growth of 1-20 nm Particles via Ozone-Human Chemistry

Dusan Licina, Shen Yang, Marouane Merizak, Meixia Zhang

Ozone reaction with human surfaces is an important source of ultrafine particles indoors. However, 1-20 nm particles generated from ozone-human chemistry, which mark the first step of particle formation and growth, remain understudied. Ventilation and indo ...

Amer Chemical Soc2024

Squalene Depletion in Skin Following Human Exposure to Ozone under Controlled Chamber Conditions

Shen Yang

A major component of human skin oil is squalene, a highly unsaturated hydrocarbon that protects the skin from atmospheric oxidants. Skin oil, and thus squalene, is continuously replenished on the skin surface. Squalene is also quickly consumed through reac ...

Amer Chemical Soc2024

New Particle Formation Events Can Reduce Cloud Droplets in Boundary Layer Clouds at the Continental Scale

Athanasios Nenes, Spyros Pandis

New particle formation (NPF) substantially contributes to global cloud condensation nuclei (CCN), and their climate impacts. Individual NPF events are also thought to increase local CCN, cloud droplet number (CDN), and cloud albedo. High resolution simulat ...

Amer Geophysical Union2024

Influence of sun cups on surface albedo of wet Alpine snowpack

Michael Lehning, Mathias Thierry Pierre Bavay, Francesca Carletti

In high elevation Alpine areas, characterised by high snow accumulation and radiation-driven melt processes, the formation of peculiar ablation features called sun cups can be observed. Sun cups likely influence the energy and mass balance of the wet snowp ...

2024

Highly Hygroscopic Aerosols Facilitate Summer and Early‐Autumn Cloud Formation at Extremely Low Concentrations Over the Central Arctic Ocean

Julia Schmale, Andrea Baccarini

Arctic clouds are sensitive to atmospheric particles since these are sometimes in such low concentrations that clouds cannot always form under supersaturated water vapor conditions. This is especially true in the late summer, when aerosol concentrations ar ...

2024

Turbulence in the Strongly Heterogeneous Near-Surface Boundary Layer over Patchy Snow

Michael Lehning, Dylan Stewart Reynolds, Michael Haugeneder

The near-surface boundary layer above patchy snow cover in mountainous terrain is characterized by a highly complex interplay of various flows on multiple scales. In this study, we present data from a comprehensive field campaign that cover a period of 21 ...

2024

Glucose Enhances Salinity-Driven Sea Spray Aerosol Production in Eastern Arctic Waters

Guangyu Li, Julia Schmale, Athanasios Nenes, André Welti

Sea spray aerosols (SSA) greatly affect the climate system by scattering solar radiation and acting as seeds for cloud droplet formation. The ecosystems in the Arctic Ocean are rapidly changing due to global warming, and the effects these changes have on t ...

2024

Atmospheric isoprene measurements reveal larger-than-expected Southern Ocean emissions

Julia Schmale, Andrea Baccarini

Isoprene is a key trace component of the atmosphere emitted by vegetation and other organisms. It is highly reactive and can impact atmospheric composition and climate by affecting the greenhouse gases ozone and methane and secondary organic aerosol format ...

Nature Research2024

Modelling the coupled mercury-halogen-ozone cycle in the central Arctic during spring

Jenny Thomas, Julia Schmale, Ivo Fabio Beck, Hélène Paule Angot

Near-surface mercury and ozone depletion events occur in the lowest part of the atmosphere during Arctic spring. Mercury depletion is the first step in a process that transforms long-lived elemental mercury to more reactive forms within the Arctic that are ...

2023

Nitrogen oxides in the free troposphere: implications for tropospheric oxidants and the interpretation of satellite NO2 measurements

Ilann Ernest Valentin Bourgeois

Satellite-based retrievals of tropospheric NO(2)columns are widely used to infer NOx (equivalent to NO + NO2) emissions. These retrievals rely on model information for the vertical distribution of NO2. The free tropospheric background above 2 km is particu ...

Copernicus GmbH2023

Arctic tropospheric ozone: assessment of current knowledge and model performance

Luca Pozzoli, Jakob Boyd Pernov, Ilann Ernest Valentin Bourgeois

As the third most important greenhouse gas (GHG) after carbon dioxide (CO2) and methane (CH4), tropospheric ozone (O3) is also an air pollutant causing damage to human health and ecosystems. This study brings together recent research on observations and mo ...

Copernicus Publications2023

Critical Review on Bromate Formation during Ozonation and Control Options for Its Minimization

Urs von Gunten

Ozone is a commonly applied disinfectant and oxidantin drinkingwater and has more recently been implemented for enhanced municipalwastewater treatment for potable reuse and ecosystem protection. Onedrawback is the potential formation of bromate, a possible ...

AMER CHEMICAL SOC2023

Assessing the simulation of snowfall at Dumont d'Urville, Antarctica, during the YOPP-SH special observing campaign

Alexis Berne, Etienne Gabriel Henri Vignon

The performance of a set of atmospheric models and meteorological reanalyses in the representation of precipitation days in Antarctica is assessed using ground-based observations such as a precipitation gauge and a Micro Rain Radar during the Year Of Polar ...

WILEY2023

Widespread detection of chlorine oxyacids in the Arctic atmosphere

Julia Schmale, Ivo Fabio Beck, Hélène Paule Angot

Observations are reported of HClO3 and HClO4 in the atmosphere and their widespread occurrence over the pan-Arctic during spring, providing further insights into atmospheric chlorine cycling in the polar environment. ...

Nature Portfolio2023

Evaluation of the role of superoxide radical as chain carrier for the formation of hydroxyl radical during ozonation

Gang Yu, Urs von Gunten, Yan Wang

Superoxide radicals (O-2(center dot-)) have been suggested as an important chain carrier in the radical chain reaction that promotes ozone (O-3) decomposition to hydroxyl radicals ((OH)-O-center dot) during ozonation. However, due to the difficulty in meas ...

PERGAMON-ELSEVIER SCIENCE LTD2023

A Case Study on Drivers of the Isotopic Composition of Water Vapor at the Coast of East Antarctica

Michael Lehning, Armin Sigmund, Riqo Chaar

Stable water isotopes (SWIs) contain valuable information on the past climate and phase changes in the hydrologic cycle. Recently, vapor measurements in the polar regions have provided new insights into the effects of snow-related and atmospheric processes ...

AMER GEOPHYSICAL UNION2023

Use of lidar aerosol extinction and backscatter coefficients to estimate cloud condensation nuclei (CCN) concentrations in the southeast Atlantic

Feng Xu, Athanasios Nenes

Accurately capturing cloud condensation nuclei (CCN) concentrations is key to understanding the aerosol-cloud interactions that continue to feature the highest uncertainty amongst numerous climate forcings. In situ CCN observations are sparse, and most non ...

COPERNICUS GESELLSCHAFT MBH2023

Investigation of the effects of the Greek extreme wildfires of August 2021 on air quality and spectral solar irradiance

In August 2021, a historic heatwave was recorded in Greece which resulted in extreme wildfire events that strongly affected the air quality over the city of Athens. Saharan dust was also transferred over Greece on certain days of the same period due to the ...

Copernicus Publications2023