Publications associées à An “ideal lignin” facilitates full biomass utilization

Development of Sustainable Carbohydrate-Based Solvents by Acetal Functionalisation of Biomass

Organic solvents are ubiquitous in industrial and domestic applications from the production of pharmaceuticals to household consumer products. The negative impact of most traditional solvents, especially aprotic types, on the environment, health, and safet ...

EPFL2024

Quantification of Native Lignin Structural Features with Gel-Phase 2D-HSQC0 Reveals Lignin Structural Changes During Extraction

Jeremy Luterbacher, Stefania Bertella

Our ability to study and valorize the lignin fraction of biomass is hampered by the fundamental and still unmet challenge of precisely quantifying native lignin's structural features. Here, we developed a rapid elevated-temperature H-1-C-13 Heteronuclear S ...

Wiley-VCH Verlag GmbH2024

Design and Synthesis of Bio-based Amphiphiles from Lignocellulosic Biomass

Songlan Sun

In the pursuit of a carbon-neutral chemical industry, minimizing fossil feedstock consumption while integrating renewable carbon sources is imperative. Surfactants, inherently amphiphilic, pose challenges in separation and recovery processes. Given their e ...

EPFL2024

Selecting Suitable Near-Native Lignins for Research

Jeremy Luterbacher

There are several methods to isolate near-native lignins, including milled-wood lignin, enzymatic lignin, cellulolytic enzyme lignin, and enzymatic mild-acidolysis lignin. Which one is the most representative of the native lignin? Herein, near-native ligni ...

Amer Chemical Soc2023

Lignin, from biomass waste to sustainable materials for food packaging, antiviral coatings and agriculture

Alice Boarino

Our planet has been challenged for years by our reckless use of fossil fuels, which has led to the ongoing climate change and energy crisis. The transition to the use of renewable alternative sources has now became urgent and inevitable. The valorization o ...

EPFL2023

Water use efficiency: A review of spatial and temporal variability

Gabriele Manoli, Sara Bonetti

Water Use Efficiency (WUE) expresses the trade-off between carbon assimilation (or subsequent carbon storage) and water release, two concurrent gas fluxes essential for plant functioning. Here, we review metrics that have been introduced to quantify WUE ac ...

Elsevier2023

Integrated production of urea and nitric acid in the pulp industry: techno-economic and environmental analysis of black liquor gasification-based processes

François Maréchal, Shivom Sharma, Daniel Alexander Florez Orrego, Meire Ellen Gorete Ribeiro Domingos

The pursuit of alternative energy sources for the nitrogen fertilizers sector has recently earned renewed interest due to increasing concerns regarding the world dependence on non-renewable energy resources and also motivated by the more stringent environm ...

2022

Biomass to energy: a machine learning model for optimum gasification pathways

Berend Smit, Kevin Maik Jablonka, Susana Garcia Lopez

Biomass is a highly versatile renewable resource for decarbonizing energy systems. Gasification is a promising conversion technology that can transform biomass into multiple energy carriers to produce heat, electricity, biofuels, or chemicals. At present, ...

Royal Soc Chemistry2023

Understanding the mechanisms of non-thermal plasma treatments on seeds

Alexandra Waskow

The motivation driving plasma-seed treatment research is the renewed importance of sustainable, eco-friendly agriculture. There is a constant interest in finding alternatives to minimize resource use and environmental degradation, while ensuring healthy se ...

EPFL2022

Time Dependent Image Generation of Plants from Incomplete Sequences with CNN-Transformer

Marc Conrad Russwurm

Data imputation of incomplete image sequences is an essential prerequisite for analyzing and monitoring all development stages of plants in precision agriculture. For this purpose, we propose a conditional Wasserstein generative adversarial network TransGr ...

SPRINGER INTERNATIONAL PUBLISHING AG2022

An optimized high throughput platform, from genetic transformation to fermentation, to screen for secreted laccases in Aspergillus niger

Laure Marie Colette Leynaud-Kieffer Curran

Many challenges are faced in the conversion of biomass into advanced biofuels, one of which is finding the correct organism for the job. The filamentous fungus Aspergillus niger has been chosen as a biocatalyst for cellulose, hemicellulose, and lignin degr ...

EPFL2021

Developing structure-oriented models for enzymatic hydrolysis of lignocellulosic biomass

Jessica Charlène Rohrbach

With the unsustainable use of fossil fuels increasing strains on human institutions and ecosystems, the development of a renewable energy alternative is of paramount importance. Second generation biorefineries, based on the production of fuels and chemical ...

EPFL2021

Toward waste valorization by converting bioethanol production residues into nanoparticles and nanocomposite films

Muhammad Farooq, Xun Liao

A "waste-valorization" approach was developed to transform recalcitrant hydrolysis lignin (HL) from secondgeneration bioethanol production into multifunctional bio-based products. The hydrolysis lignin (HL) was extracted with aqueous acetone, yielding two ...

ELSEVIER2021

Techno-economic analysis and life cycle assessment of a biorefinery utilizing reductive catalytic fractionation

Jeremy Luterbacher

Reductive catalytic fractionation (RCF) is a promising approach to fractionate lignocellulose and convert lignin to a narrow product slate. To guide research towards commercialization, cost and sustainability must be considered. Here we report a techno-eco ...

2021

Aldehyde-Assisted Lignocellulose Fractionation Provides Unique Lignin Oligomers for the Design of Tunable Polyurethane Bioresins

Jeremy Luterbacher, Raymond Gérard Buser, Florent Emmanuel Héroguel, Jean Thierry C Behaghel de Bueren, Chloé Wegmann

Thanks to chemical stabilization, aldehyde-assisted fractionation (AAF) of lignocellulosic biomass has recently emerged as a powerful tool for the production of largely uncondensed lignin. Depolymerization of AAF lignin via ether deavage provides aromatic ...

American Chemical Society2020

Lignin Functionalization for the Production of Novel Materials

Jeremy Luterbacher, Stefania Bertella

Lignin, a major constituent of lignocellulosic biomass, is the largest natural source of aromatic molecules and thus is an attractive feedstock for renewable chemical production. Direct incorporation of isolated lignin into materials has long been research ...

2020

Production and characterization of stabilized lignin

Masoud Talebi Amiri

Lignocellulosic biomass is a sustainable source of renewable carbon, and it is the most abundant form of terrestrial biomass. The three main constituents of lignocellulosic biomass are cellulose, hemicellulose, and lignin. The monomers from these biopolyme ...

EPFL2019

Enzymes for second generation biofuels: recent developments and future perspectives

Edgard Gnansounou, Binod Parameswaran

Even though the search for alternative fuels from lignocellulosic biomass started a few decades ago, still it is relatively immature mainly because of few challenges which are yet to be solved for making the process commercially viable. The main challenge ...

2019

Topology of Pretreated Wood Fibers Using Dynamic Nuclear Polarization

Jeremy Luterbacher, Arthur César Pinon, David Lyndon Emsley, Jasmine Viger-Gravel, Wu Lan, Michel Bardet, Pierrick Berruyer

In the continuously developing field of lignocellulosic biomass, high-yield lignin depolymerization processes are sought to optimize its productivity and profitability. Recently, formaldehyde stabilization during lignin extraction and biomass pretreatment ...

2019

Fractionation of lignocellulosic biomass to produce uncondensed aldehyde-stabilized lignin

Jeremy Luterbacher, Masoud Talebi Amiri, Ydna Marie Questell-Santiago, Graham Reid Dick

Lignin is one of the most promising sources of renewable aromatic hydrocarbons. Current methods for its extraction from lignocellulosic biomass—which include the kraft, sulfite, and organosolv processes—result in the rapid formation of carbon–carbon bonds, ...

2019