Publications associées à Dissolved Organic Matter and Associated Trace Metal Dynamics from River to Lake, Under Ice-Covered and Ice-Free Conditions

Treeline displacement may affect lake dissolved organic matter processing at high latitudes and altitudes

Climate change induced shifts in treeline position, both towards higher altitudes and latitudes induce changes in soil organic matter. Eventually, soil organic matter is transported to alpine and subarctic lakes with yet unknown consequences for dissolved ...

Nature Portfolio2024

Adsorption of Copper by Naturally and Artificially Aged Polystyrene Microplastics and Subsequent Release in Simulated Gastrointestinal Fluid

Florian Frédéric Vincent Breider, Thibault Béranger Masset, Lu Zhou

Microplastics, especially aged microplastics can become vectors of metals from environment to organisms with potential negative effects on food chain. However, a few studies focused on the bioavailability of adsorbed metals and most studies related to aged ...

2024

Characteristics and sources of fluorescent aerosols in the central Arctic Ocean

Benjamin Jérémy Laurent Heutte, Julia Schmale, Ivo Fabio Beck, Margarida Teles Nogueira Rolo, Hélène Paule Angot, Oliver Müller, Jakob Boyd Pernov, Nora Bergner, Alireza Moallemi, Markus Frey

The Arctic is sensitive to cloud radiative forcing. Due to the limited number of aerosols present throughout much of the year, cloud formation is susceptible to the presence of cloud condensation nuclei and ice nucleating particles (INPs). Primary biologic ...

2024

Glucose Enhances Salinity-Driven Sea Spray Aerosol Production in Eastern Arctic Waters

Guangyu Li, Julia Schmale, Athanasios Nenes, André Welti

Sea spray aerosols (SSA) greatly affect the climate system by scattering solar radiation and acting as seeds for cloud droplet formation. The ecosystems in the Arctic Ocean are rapidly changing due to global warming, and the effects these changes have on t ...

2024

Oxidation processes and me

Urs von Gunten

This publication summarizes my journey in the field of chemical oxidation processes for water treatment over the last 30+ years. Initially, the efficiency of the application of chemical oxidants for micropollutant abatement was assessed by the abatement of ...

Pergamon-Elsevier Science Ltd2024

Photo-Fenton inactivation of MS2 bacteriophage at alkaline pH by Fe salts or nm to μm-sized oxides, and the Janus-faced effects of natural organic matter in surface waters

César Pulgarin, Stefanos Giannakis, Ogadimma Cassandra Oji-Okoro, Giulio Farinelli

In this study, MS2 bacteriophage was inactivated by homogeneous and heterogeneous photo-Fenton processes in an alkaline matrix (pH 8) using low concentrations of H2O2 and iron forms (1 mg/L), including Fe(II), Fe(III), and Fe (hydr)oxides. As a reference, ...

Elsevier2024

Organic matters, but inorganic matters too: column examination of elevated mercury sorption on low organic matter aquifer material using concentrations and stable isotope ratios

Lorenz Schwab

Sorption of mercury (Hg) in soils is suggested to be predominantly associated with organic matter (OM). However, there is a growing collection of research that suggests that clay minerals and oxides are also important solid phases for the sorption of solu ...

2024

The molecular scale mechanism of deposition ice nucleation on silver iodide

Mária Lbadaoui-Darvas, Athanasios Nenes, André Welti

Heterogeneous ice nucleation is a ubiquitous process in the natural and built environment. Deposition ice nucleation, i.e. heterogeneous ice nucleation that - according to the traditional view - occurs in a subsaturated water vapor environment and in the a ...

Royal Soc Chemistry2024

CRYOWRF—Model Evaluation and the Effect of Blowing Snow on the Antarctic Surface Mass Balance

Michael Lehning, Varun Sharma, Franziska Gerber

The surface mass balance (SMB) of large polar ice sheets and of snow and ice surfaces in general are incompletely understood because of the complexity of processes involved. One such process, drifting and blowing snow, has only been considered in a very si ...

AMER GEOPHYSICAL UNION2023

Blue ice in Antarctica: The gateway to travel in time and space

Devis Tuia, Benjamin Alexander Kellenberger, Marc Conrad Russwurm, Veronica Tollenaar

Antarctica has unique areas that expose blue ice, which contrast to most of the continent (~98%) that is covered by snow. Some of these blue ice areas (BIAs) contain meteorite concentrations and (very) old ice, making them very valuable for understanding o ...

GFZ German Research Centre for Geosciences2023

Near-bed stratification controls bottom hypoxia in ice-covered alpine lakes

Damien Bouffard, Pascal Perolo, Tomy Doda, Nicolas Thomas Georges Escoffier, Janine Rüegg, Hannah Elisa Chmiel, Hugo Nicolás Ulloa Sánchez, Camille Roland Marie Minaudo

In ice-covered lakes, near-bottom oxygen concentration decreases for most of the wintertime, sometimes down to the point that bottom waters become hypoxic. Studies insofar have reached divergent conclusions on whether climate change limits or reinforces th ...

American Society of Limnology and Oceanography2023

A full year of aerosol size distribution data from the central Arctic under an extreme positive Arctic Oscillation: insights from the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition

Benjamin Jérémy Laurent Heutte, Federico Bianchi, Julia Schmale, Ivo Fabio Beck, Lubna Dada, Hélène Paule Angot, Jakob Boyd Pernov

The Arctic environment is rapidly changing due to accelerated warming in the region. The warming trend is driving a decline in sea ice extent, which thereby enhances feedback loops in the surface energy budget in the Arctic. Arctic aerosols play an importa ...

Copernicus Publications2023

Polar oceans and sea ice in a changing climate

Jenny Thomas, Julia Schmale, Hélène Paule Angot

Polar oceans and sea ice cover 15% of the Earth’s ocean surface, and the environment is changing rapidly at both poles. Improving knowledge on the interactions between the atmospheric and oceanic realms in the polar regions, a Surface Ocean–Lower Atmospher ...

2023

Spatio-Temporal Dynamics of Snow on Central Arctic Sea Ice and its Implications

David Nicholas Wagner

This thesis presents a comprehensive investigation of the interaction between precipitation and wind-induced erosion and deposition of snow on Arctic sea ice. The study uses observations from the 2019-2020 MOSAiC expedition and makes use of the 3D snow cov ...

EPFL2023

Physicochemical characterization and source apportionment of Arctic ice-nucleating particles observed in Ny-Alesund in autumn 2019

Guangyu Li, Athanasios Nenes, Jörg Wieder, Ghislain Gilles Jean-Michel Motos

Ice-nucleating particles (INPs) initiate primary ice formation in Arctic mixed-phase clouds (MPCs), altering cloud radiative properties and modulating precipitation. For atmospheric INPs, the complexity of their spatiotemporal variations, heterogeneous sou ...

Copernicus GmbH2023

Low ozone dry deposition rates to sea ice during the MOSAiC field campaign: Implications for the Arctic boundary layer ozone budget

Julia Schmale, Ivo Fabio Beck, Hélène Paule Angot

Dry deposition to the surface is one of the main removal pathways of tropospheric ozone (O3). We quantified for the first time the impact of O3 deposition to the Arctic sea ice on the planetary boundary layer (PBL) O3 concentration and budget using year-ro ...

2023

The role of secondary ice production in mixed-phase clouds

Paraskevi Georgakaki

Clouds are omnipresent in the Earth's atmosphere. Their phase composition significantly modulates their interaction with solar and terrestrial radiation, as well as precipitation formation. Particularly for clouds containing both phases, known as mixed-pha ...

EPFL2023

Reactivity of Bromine Radical with Dissolved Organic Matter Moieties and Monochloramine: Effect on Bromate Formation during Ozonation

Urs von Gunten, Sung Eun Lim

Bromine radical (Br center dot) has been hypothesized to be a key intermediate of bromate formation during ozonation. Once formed, Br center dot further reacts with ozone to eventually form bromate. However, this reaction competes with the reaction of Br c ...

AMER CHEMICAL SOC2023

The biofilm ecology of proglacial floodplain streams

Jade Brandani

Glacial forelands figure among the most dynamic landscapes on Earth, and their formation is currently accelerating given glacier shrinkage. Draining these forelands are streams hosting unique microbial communities, which have the capacity to impact both th ...

EPFL2023

Improving algal bloom detection using spectroscopic analysis and machine learning: A case study in a large artificial reservoir, South Korea

Trung-Dung Hoang, Thanh Trung Huynh

The prediction of algal blooms using traditional water quality indicators is expensive, labor-intensive, and timeconsuming, making it challenging to meet the critical requirement of timely monitoring for prompt management. Using optical measures for foreca ...

ELSEVIER2023