Publications associées à Disorder and Halide Distributions in Cesium Lead Halide Nanocrystals as Seen by Colloidal 133Cs Nuclear Magnetic Resonance Spectroscopy

Treeline displacement may affect lake dissolved organic matter processing at high latitudes and altitudes

Climate change induced shifts in treeline position, both towards higher altitudes and latitudes induce changes in soil organic matter. Eventually, soil organic matter is transported to alpine and subarctic lakes with yet unknown consequences for dissolved ...

Nature Portfolio2024

Excess labile carbon promotes diazotroph abundance in heat-stressed octocorals

Claudia Isabella Pogoreutz

Nitrogen limitation is the foundation of stable coral-algal symbioses. Diazotrophs, prokaryotes capable of fixing N-2 into ammonia, support the productivity of corals in oligotrophic waters, but could contribute to the destabilization of holobiont function ...

ROYAL SOC2023

What happens to biomass burning-emitted particles in the ocean? A laboratory experimental approach based on their tracers

Christos Panagiotopoulos

Wildfires, controlled burns, and biofuel combustion (biomass burning or BB) are major contributors to particulate matter in the atmosphere and thus have an impact on climate, human health, and ecosystems. Once emitted, the particulate matter derived from B ...

Elsevier2023

High-Throughput Sizing, Counting, and Elemental Analysis of Anisotropic Multimetallic Nanoparticles with Single-Particle Inductively Coupled Plasma Mass Spectrometry

Natalia Gasilova, Andreas Züttel, Wen Luo, Mo Li, Cedric David Koolen, Ayush Agarwal

Nanoparticles (NPs) have wide applications in physical and chemical processes, and their individual properties (e.g., shape, size, and composition) and ensemble properties (e.g., distribution and homogeneity) can significantly affect the performance. Howev ...

2022

Glacier shrinkage will accelerate downstream decomposition of organic matter and alters microbiome structure and function

Nicola Deluigi, Leïla Ezzat, Vincent Henri De Staercke, Tom Ian Battin, Paraskevi Pramateftaki, Hannes Markus Peter, Jade Brandani, Matteo Tolosano, Michail Styllas, Tyler Joe Kohler, Stylianos Fodelianakis, Massimo Bourquin, Martina Andrea Schön, Susheel Bhanu Busi, Grégoire Marie Octave Edouard Michoud

The shrinking of glaciers is among the most iconic consequences of climate change. Despite this, the downstream consequences for ecosystem processes and related microbiome structure and function remain poorly understood. Here, using a space-for-time substi ...

Wiley2022

Contrasting Microbiome Dynamics of Putative Denitrifying Bacteria in Two Octocoral Species Exposed to Dissolved Organic Carbon (DOC) and Warming

Nils Rädecker, Claudia Isabella Pogoreutz

Mutualistic nutrient cycling in the coral-algae symbiosis depends on limited nitrogen (N) availability for algal symbionts. Denitrifying prokaryotes capable of reducing nitrate or nitrite to dinitrogen could thus support coral holobiont functioning by limi ...

2022

Detritus-hosted methanogenesis sustains the methane paradox in an alpine lake

Damien Bouffard, Oscar Rodrigo Sepúlveda Steiner

Accumulation of methane in oxic waters of lakes and the ocean has been widely reported. Despite the importance for the greenhouse gas budget, mechanistic controls of such "methane paradox" remain elusive. Here, we use a combination of CH4 concentration and ...

American Society of Limnology and Oceanography2022

Synthesizing the impacts of baseflow contribution on concentration-discharge (C-Q) relationships across Australia using a Bayesian hierarchical model

Camille Roland Marie Minaudo

Understanding concentration-discharge (C - Q) relationships can inform catchment solute and particulate export processes. Previous studies have shown that the extent to which baseflow contributes to streamflow can affect C-Q relationships in some catchment ...

COPERNICUS GESELLSCHAFT MBH2022

Low and high frequency electromagnetic forces: numerical modelling and practical applications

Marco Riccardi

The understanding and manipulation of nanoscale analytes is a central theme in nanotechnology and has been one of the main driving forces behind the development of this field as we know it today. Furthermore, such a technology has the potential to also rev ...

EPFL2022

Reaction of DMS and HOBr as a Sink for Marine DMS and an Inhibitor of Bromoform Formation

Boris Droz, Urs von Gunten

Recently, we suggested that hypobromous acid (HOBr) is a sink for the marine volatile organic sulfur compound dimethyl sulfide (DMS). However, HOBr is also known to react with reactive moieties of dissolved organic matter (DOM) such as phenolic compounds t ...

2021

Cu/Metal Oxide Hybrid Nanocrystals as Electrocatalysts for the CO2 Reduction Reaction

Seyedehbehnaz Varandili

The electrochemical CO2 reduction reaction (CO2RR) is envisioned to play a significant role in achieving carbon neutrality while contributing to storing renewable energies. Cu-based materials are among the most promising electrocatalysts. However, 16 diffe ...

EPFL2021

Heterotrophy in the earliest gut: a single-cell view of heterotrophic carbon and nitrogen assimilation in sponge-microbe symbioses

Anders Meibom, Stéphane Laurent Escrig

Sponges are the oldest known extant animal-microbe symbiosis. These ubiquitous benthic animals play an important role in marine ecosystems in the cycling of dissolved organic matter (DOM), the largest source of organic matter on Earth. The conventional vie ...

NATURE PUBLISHING GROUP2020

Travel Time and Source Variation Explain the Molecular Transformation of Dissolved Organic Matter in an Alpine Stream Network

Tom Ian Battin, Amber Joy Ulseth, Hannes Markus Peter

Streams and rivers are important components of the carbon cycle as they transport and transform dissolved organic matter (DOM). Using high resolution Fourier transform ion cyclotron resonance mass spectrometry, we studied the spatial distribution of DOM at ...

2020

Delineating the Continuum of Dissolved Organic Matter in Temperate River Networks

Luis Gómez Gener

The origin and reactivity of dissolved organic matter (DOM) have received attention for decades due to the key role DOM plays in global carbon cycling and the ecology of aquatic systems. However, DOM dynamics in river networks remain unresolved, hampered b ...

2020

Predicting the reflectivity and colour of metals from first principles

Gianluca Prandini

Gold and copper are the only two elemental metals that show a characteristic colour, due to the presence of a drop in the reflectivity curve inside the visible range. Reflectivities of all other metals are in general high and flat for all visible frequenci ...

EPFL2019

Dissolved Organic Nitrogen Production and Export by Meridional Overturning in the Eastern Subpolar North Atlantic

Bieito Fernandez Castro

Dissolved organic matter (DOM) is produced in the surface and exported towards the deep ocean, adding similar to 2 PgC/year to the global carbon export. Due to its central role in the Meridional Overturning Circulation, the eastern subpolar North Atlantic ...

2019

Designing high ductility in magnesium alloys

William Curtin, Zhaoxuan Wu, Binglun Yin, Rasool Ahmad

The thermally activated pyramidal-to-basal (PB) transition of (c + a) dislocations, transforming glissile pyramidal dissociated core structures into sessile basal dissociated ones, lies at the origin of low ductility in pure magnesium (Mg). Solute-accelera ...

PERGAMON-ELSEVIER SCIENCE LTD2019

Colloidal Size and Redox State of Uranium Species in the Porewater of a Pristine Mountain Wetland

Rizlan Bernier-Latmani, Manon Frutschi, Barbora Bártová, Giada Chantal Zünd, Gabrielle Dublet, Ashley Richards Brown

Uranium (U) speciation was investigated in anoxically preserved porewater samples of a natural mountain wetland in Gola di Lago, Ticino, Switzerland. U porewater concentrations ranged from less than 1 mu g/L to tens of mu g/L, challenging the available ana ...

AMER CHEMICAL SOC2019

Density effects on nanoparticle transport in the hyporheic zone

David Andrew Barry, Ho Ling Li, Qihao Jiang

A carbon solution composed of nanoparticles was used in experiments designed to explore nanoparticle transport characteristics within the hyporheic zone of a riverbed. Experiments and numerical simulations demonstrated that nanoparticle transport in the hy ...

2018

Creation of Faceted Polyhedral Microgels from Compressed Emulsions

Jing Fan, Esther Amstad

Compressed monodisperse emulsions in confined space exhibit highly ordered structures. The influence of the volume fraction and the confinement geometry on the organized structures is investigated and the mechanism by which structural transition occurs is ...

Wiley-V C H Verlag Gmbh2017