Publication

Phonons, electron-phonon coupling and charge transport in low-dimensional materials

Publications associées (20)

Long-range electrostatic contribution to electron-phonon couplings and mobilities of two-dimensional and bulk materials

Massimiliano Stengel, Nicola Marzari, Marco Gibertini, Samuel Poncé

Charge transport plays a crucial role in manifold potential applications of two-dimensional materials, in-cluding field-effect transistors, solar cells, and transparent conductors. At most operating temperatures, charge transport is hindered by scattering ...

AMER PHYSICAL SOC2023

Resonant Inelastic X-Ray Scattering Study of Electron-Exciton Coupling in High-T-c Cuprates

Christophe Berthod, Fabrizio Carbone, Ivan Madan, Yi Tseng, Francesco Barantani, Thorsten Schmitt, Dirk Van der Marel

Explaining the mechanism of superconductivity in the high-T-c cuprates requires an understanding of what causes electrons to form Cooper pairs. Pairing can be mediated by phonons, the screened Coulomb force, spin or charge fluctuations, excitons, or by a c ...

American Physical Society2022

Time- and Angle-Resolved Photoelectron Spectroscopy of Solar Materials

Serhii Polishchuk

Natural foundations defining the manner in which a solid material interacts with optical radiation are primarily encoded in the material's momentum-dependent band structure and the microscopic details of the electron-lattice interactions. An access to this ...

EPFL2021

Evidence of a coupled electron-phonon liquid in NbGe2

Mathieu François Padlewski, Philip Johannes Walter Moll, Matthias Carsten Putzke, Hao Yang

Whereas electron-phonon scattering relaxes the electron's momentum in metals, a perpetual exchange of momentum between phonons and electrons may conserve total momentum and lead to a coupled electron-phonon liquid. Such a phase of matter could be a platfor ...

Nature Portfolio2021

Electron-phonon-driven three-dimensional metallicity in an insulating cuprate

Cédric Weber, Fabrizio Carbone, Edoardo Baldini

The role of the crystal lattice for the electronic properties of cuprates and other high-temperature superconductors remains controversial despite decades of theoretical and experimental efforts. While the paradigm of strong electronic correlations suggest ...

National Academy of Sciences2020

Nonequilibrium exciton physics in hybrid lead-halide perovskites and anatase titanium dioxide

Tania Palmieri

The strength of the electron-hole interaction in bulk semiconductors is not only determined by the dielectric environment, but also depends on the presence of other quasiparticles - free charge carriers or phonons - that populate the system. In the former ...

EPFL2019

Valley-Engineering Mobilities in Two-Dimensional Materials

Nicola Marzari, Giovanni Pizzi, Marco Gibertini, Thibault Daniel Pierre Sohier, Davide Campi

Two-dimensional materials are emerging as a promising platform for ultrathin channels in field-effect transistors. To this aim, novel high-mobility semiconductors need to be found or engineered. Although extrinsic mechanisms can in general be minimized by ...

AMER CHEMICAL SOC2019

Electric field exfoliation and high-T-C superconductivity in field-effect hole-doped hydrogenated diamond (111)

Thibault Daniel Pierre Sohier

We investigate the possible occurrence of field-effect induced superconductivity in the hydrogenated (111) diamond surface by first-principles calculations. By computing the band alignment between bulk diamond and the hydrogenated surface, we show that the ...

2019

Crystalline and correlated phases in two-dimensional transition metal dichalcogenides

Diego José Pasquier

This thesis is dedicated to the study of various aspects of the electronic structure of two-dimensional transition metal dichalcogenides (TMDs) of chemical composition MX

_2

(where M is a transition metal atom and X= S, Se, Te), using a combination of \te ...

EPFL2019

Mobility of two-dimensional materials from first principles in an accurate and automated framework

Nicola Marzari, Marco Gibertini, Thibault Daniel Pierre Sohier, Davide Campi

We present a first-principles approach to compute the transport properties of 2D materials in an accurate and automated framework. We use density-functional perturbation theory in the appropriate bidimensional setup with open-boundary conditions in the thi ...

AMER PHYSICAL SOC2018

Defect chemistry of methylammonium lead iodide

Alessandro Senocrate

The present work deals with the defect chemistry and charge transport properties in halide perovskites, and in particular in the archetypal methylammonium lead iodide. These materials are extensively researched due to their very promising application as li ...

EPFL2018

A Time-Resolved Photophysical Study of Hybrid Organic-Inorganic Perovskite Photovoltaic Materials

Arun Aby Paraecattil

The search for new photovoltaic materials has been driven by the combined need to exploit sources of energy that are clean and sustainable, while simultaneously doing it in a cost effective manner. In this light, hybrid organic-inorganic perovskites have r ...

EPFL2017

Two-dimensional Frohlich interaction in transition-metal dichalcogenide monolayers: Theoretical modeling and first-principles calculations

Thibault Daniel Pierre Sohier

We perform ab initio calculations of the coupling between electrons and small-momentum polar-optical phonons in monolayer transition-metal dichalcogenides of the 2H type: MoS2, MoSe2, MoTe2, WS2, and WSe2. The polar-optical coupling with longitudinal optic ...

Amer Physical Soc2016

Thermal transport in low dimensions

Andrea Cepellotti

Lattice vibrations are the microscopic mechanism responsible for a large, if not dominant, contribution to heat transport in crystalline insulators. These vibrations are described in terms of phonons, collective excitations (or quasiparticles) in the form ...

EPFL2016

Dissociation of charge transfer states and carriers separation in bilayer organic solar cells - A time-resolved electroabsorption spectroscopy study

Jacques-Edouard Moser, Jelissa Risse, Roland Hany

Ultrafast optical probing of the electric field by means of Stark effect in planar heterojunction cyanine dye / fullerene organic solar cells enables to directly monitor the dynamics of free electron formation during the dissociation of interfacial charge ...

Amer Chemical Soc2015

Electron-Phonon Interactions and the Intrinsic Electrical Resistivity of Graphene

Nicola Marzari, Boris Kozinsky, Thibault Daniel Pierre Sohier

We present a first-principles study of the temperature- and density-dependent intrinsic electrical resistivity of graphene. We use density-functional theory and density-functional perturbation theory together with very accurate Wannier interpolations to co ...

Amer Chemical Soc2014

Self-energy effects and electron-phonon coupling in Fe-As superconductors

Helmuth Berger

Doping and temperature dependent studies of optical phonon modes in Fe-122 pnictides are performed using Raman scattering experiments and compared with model calculations to elucidate the role of electron-phonon and spin-phonon interaction in this family o ...

2010

Electron-phonon interaction and charge carrier mass enhancement in SrTiO3

Claudio Grimaldi, Dirk Van der Marel

We report a comprehensive THz, infrared and optical study of Nb-doped SrTiO3 as well as dc conductivity and Hall effect measurements. Our THz spectra at 7 K show the presence of an unusually narrow (< 2 meV) Drude peak. For all carrier concentrations the D ...

2008

Trapping, self-trapping and the polaron family

Henrik Moodysson Rønnow

The earliest ideas of the polaron recognized that the coupling of an electron to ionic vibrations would affect its apparent mass and could effectively immobilize the carrier (self-trapping). We discuss how these basic ideas have been generalized to recogni ...

IOP PUBLISHING LTD2007

Transistors organiques ultraminces à base de pentacène

Adrian von Mühlenen

The goal of this thesis is to contribute to the understanding of charge transport in organic field-effect transistors (OFETs) made of pentacene. Organic thin-film transistors (OTFTs) with active layers thicknesses of 5, 10, 20, and 100 nm were fabricated i ...

EPFL2007

Publications associées (20)

_2

(where M is a transition metal atom and X= S, Se, Te), using a combination of \te ...

EPFL2019

Two-dimensional Frohlich interaction in transition-metal dichalcogenide monolayers: Theoretical modeling and first-principles calculations

Thibault Daniel Pierre Sohier

Amer Physical Soc2016

Thermal transport in low dimensions

Andrea Cepellotti

EPFL2016

Dissociation of charge transfer states and carriers separation in bilayer organic solar cells - A time-resolved electroabsorption spectroscopy study

Jacques-Edouard Moser, Jelissa Risse, Roland Hany

Amer Chemical Soc2015