Publications associées à LaTiO2N/In2O3 photoanodes with improved performance for solar water splitting

Stability and degradation of (oxy)nitride photocatalysts for solar water splitting

Sophia Haussener, Franky Esteban Bedoya Lora

Advancing towards alternative technologies for the sustainable production of hydrogen is a necessity for the successful integration of this potentially green fuel in the future. Photocatalytic and photoelectrochemical water splitting are promising concepts ...

2024

Data-Intensive Exploration of the Photoelectrochemical Responses of Main-Group Metal Sulfides

Nicola Colonna

Materials that efficiently promote the thermodynamically uphill water-splitting reaction under solar illumination are essential for generating carbon-free ("green") hydrogen. Mapping out the combinatorial space of potential photocatalysts for this reaction ...

Amer Chemical Soc2024

Single emulsion drops for photocatalytic water splitting as a membrane-free approach to product separation

Sophia Haussener, Esther Amstad, Swarnava Nandy, Sangram Ashok Savant, Gaia De Angelis

The coevolution of hydrogen and oxygen during photocatalytic water splitting presents a challenge for efficient product separation. Here, we demonstrate membrane-free, drop-based photocatalytic water splitting with inherent product separation and competiti ...

2023

Photoelectrochemical Cell Engineering for Solar Energy Conversion

Dan Zhang

Solar energy is the most abundant energy source, harnessing solar energy holds the solution to the challenge of increasing global energy demand and reducing our dependence on fossil fuels. Photovoltaics which directly convert solar energy into electricity ...

EPFL2023

Radiation Hardness of MALTA2, a Monolithic Active Pixel Sensor for Tracking Applications

Edoardo Charbon, Ashish Sharma, Francesco Piro

MALTA is a depleted monolithic active pixel sensor (DMAPS) developed in the Tower Semiconductor 180-nm CMOS imaging process. Monolithic CMOS sensors offer advantages over current hybrid imaging sensors in terms of both increased tracking performance due to ...

Ieee-Inst Electrical Electronics Engineers Inc2023

Solar Water Splitting Using Earth-Abundant Electrocatalysts Driven by High-Efficiency Perovskite Solar Cells

Michael Graetzel, Shaik Mohammed Zakeeruddin, Dan Ren, Hong Zhang

Hydrogen is considered as the "holy grail" for the energy community. One of the most promising strategies to produce hydrogen is to split water using renewable energy such as solar radiation. The abundance of water and solar energy enables the potential of ...

WILEY-V C H VERLAG GMBH2022

Engineering of PEM-PEC photocathodes for solar-driven hydrogen production

Marina Caroline Michèle Caretti

Earth has always been in perpetual evolution, but today we must face its rapid change due to human activity. The intensification of industrial activities and transportation to support our modern lifestyles are the main causes of climate change and the adve ...

EPFL2022

Modeling the Photostability of Solar Water-Splitting Devices and Stabilization Strategies

Sophia Haussener, Fredy Intelligent Nandjou Dongmeza

The practical implementation of photoelectrochemical devices for hydrogen generation is limited by their short lifetimes. Understanding the factors affecting the stability of the heterogeneous photoelectrodes is required to formulate degradation mitigation ...

2022

Novel Interfacial Characterization and Surface Engineering in Semiconductor Electrodes for Optimized Solar Fuel Production

Yongpeng Liu

Harvesting sunlight, the ultimate renewable power source, in a cost-effective way has been long recognized as a necessary route to meet the global energy challenges. Solar energy can be transformed into electricity by means of photovoltaic devices to suppl ...

EPFL2021

Prospects and challenges in designing photocatalytic particle suspension reactors for solar fuel processing

Sophia Haussener, Swarnava Nandy, Sangram Ashok Savant

Photocatalytic approaches for the production of solar hydrogen or hydrocarbons are interesting as they provide a sustainable alternative to fossil fuels. Research has been focused on water splitting and on the synthesis of photocatalyst materials and compo ...

2021

Spray Synthesis of CuFeO2 Photocathodes and In-Operando Assessment of Charge Carrier Recombination

Kevin Sivula, Florian Le Formal, Nestor Guijarro Carratala, Yongpeng Liu, Florent Alexandre Boudoire, Charles Roger Jean Lhermitte

Semiconducting delafossite-phase CuFeO2 is a promising photocathode material for solar-driven hydrogen production given its suitable energy levels and established robustness for photoelectrochemical water reduction. Nevertheless, reported methods for prepa ...

AMER CHEMICAL SOC2021

Understanding Surface Recombination Processes Using Intensity-Modulated Photovoltage Spectroscopy on Hematite Photoanodes for Solar Water Splitting

Kevin Sivula, Nestor Guijarro Carratala, Yongpeng Liu

Converting solar energy into hydrogen through photoelectrochemical (PEC) water splitting offers a promising route towards a fully renewable energy economy. A fundamental understanding of photogenerated charge recombination processes in semiconducting photo ...

WILEY-V C H VERLAG GMBH2020

Strategies for Semiconductor/Electrocatalyst Coupling toward Solar-Driven Water Splitting

Xile Hu, Lichen Bai, Lei Liu

Hydrogen (H-2) has a significant potential to enable the global energy transition from the current fossil-dominant system to a clean, sustainable, and low-carbon energy system. While presently global H-2 production is predominated by fossil-fuel feedstocks ...

2020

Mitigating voltage losses in photoelectrochemical cell scale-up

Sophia Haussener, Ronald Ramiro Gutierrez Perez

In solar water splitting, efforts in scaling up the photoelectrochemical cell beyond laboratory scale have started to attract significant attention. Several large-area devices have been demonstrated, but typically the efficiencies are much lower than their ...

ROYAL SOC CHEMISTRY2020

Synthesis of metal oxide photoanodes for water splitting using nanocrystals as precursors

Chethana Janardhana Gadiyar

Photoelectrochemical (PEC) water splitting devices are envisioned to play a key role in the societal transition towards sustainable energy sources. In this context, multinary metal oxide semiconductors are the most promising candidates for the role of phot ...

EPFL2020

Containergy-A Container-Based Energy and Performance Profiling Tool for Next Generation Workloads

David Atienza Alonso, Marina Zapater Sancho, Arman Iranfar, Wellington Silva De Souza

Run-time profiling of software applications is key to energy efficiency. Even the most optimized hardware combined to an optimally designed software may become inefficient if operated poorly. Moreover, the diversification of modern computing platforms and ...

2020

Multidimensional Measures of Physical Activity and Their Association with Gross Motor Capacity in Children and Adolescents with Cerebral Palsy

Anisoara Ionescu, Lena Carcreff, Stéphane Armand

The current lack of adapted performance metrics leads clinicians to focus on what children with cerebral palsy (CP) do in a clinical setting, despite the ongoing debate on whether capacity (what they do at best) adequately reflects performance (what they d ...

2020

Exploring Perovskite-Metal Nanoassemblies for Photocatalytic Applications

Seryio Saris

The development of sustainable, renewable and economic chemical processes lies in the centre of todayâ s global energy challenge. Like in plants, artificial photosynthesis offers an auspicious solution in harvesting solar energy and storing it in chemical ...

EPFL2020

Measurement-system design for structural identification

Numa Joy Bertola

In developed countries, the management of existing civil infrastructure is challenging due to evolving functional requirements, aging and climate change. Due to conservative approaches in construction design and practice, infrastructure often has hidden re ...

EPFL2020

Solar Water Splitting with Perovskite/Silicon Tandem Cell and TiC-Supported Pt Nanocluster Electrocatalyst

Christophe Ballif, Michael Graetzel, Shaik Mohammed Zakeeruddin, Quentin Thomas Jeangros, Jérémie Werner, Florent Sahli, Jingshan Luo, Dan Ren, Jing Gao

Developing efficient, stable, and cost-effective photosystems to split water into hydrogen and oxygen using sunlight is of paramount importance for future production of fuels and chemicals from renewable sources. However, the high cost of current systems l ...

2019