Publications associées à Uranium de retraitement

Atomic level insight into irradiation effects in nuclear fuel materials

Microstructural evolution during in-pile irradiation, radiation damage effects and fission products behavior in UO2 nuclear fuel are key issues in understanding and for the modeling of the performance as well as safety characteristics of nuclear fuels in t ...

EPFL2024

Biostimulation as a sustainable solution for acid neutralization and uranium immobilization post acidic in-situ recovery

Rizlan Bernier-Latmani, Pierre Rossi, Thomas Coral

Major uranium (U) deposits worldwide are exploited by acid leaching, known as 'in-situ recovery' (ISR). ISR involves the injection of an acid fluid into ore-bearing aquifers and the pumping of the resulting metal-containing solution through cation exchange ...

2022

Interface Tracking Investigation of the Sliding Bubbles Effects on Heat Transfer in the Laminar Regime

Konstantin Mikityuk, Lubomír Bures

Helium gases are utilized to remove fission products from the molten salt fast reactor (MSFR) core during operation. Helium gases and other volatile fission products may be introduced into the intermediate heat exchanger channels. The effect of these gases ...

2022

Structural performance and mechanical properties investigation of spent nuclear fuel rods under static and dynamic bending loads

Efstathios Vlassopoulos

Currently, most Spent Nuclear Fuel (SNF) is kept safely in storage either at on-site facilities or at centralized interim storage sites. Moreover, many countries face delays in implementing their waste management programmes for SNF and high-level waste dis ...

EPFL2021

Applying SHARK-X to perform data assimilation with the LWR-PROTEUS Phase II integral experiments

Andreas Pautz, Daniel Jerôme Siefman, Mathieu Hursin

Data assimilation methods have recently been implemented in the sensitivity analysis and uncertainty quantification tool SHARK-X. This paper presents how they were used with sensitivity coefficients and randomly-sampled nuclear data to simulate integral pa ...

PERGAMON-ELSEVIER SCIENCE LTD2020

Nanoscale mechanism of UO2 formation through uranium reduction by magnetite

Rizlan Bernier-Latmani, Barbora Bártová, Thomas La Grange, Zezhen Pan

Uranium (U) is a ubiquitous element in the Earth's crust at similar to 2 ppm. In anoxic environments, soluble hexavalent uranium (U(VI)) is reduced and immobilized. The underlying reduction mechanism is unknown but likely of critical importance to explain ...

Nature Research2020

Statistical Burnup Distribution of Moving Pebbles in the High-Temperature Reactor HTR-PM

Andreas Pautz, Jiri Krepel, Fanny Vitullo, Horst-Michael Prasser

In the pebble-bed high-temperature reactor under construction in China, called the HTR-PM, the spherical fuel elements continuously flow downward in the cylindrical core. The burnup of each pebble is checked at the core outlet and, according to the achieve ...

ASME2020

Loading optimization for Swiss used nuclear fuel assemblies into final disposal canisters

Andreas Pautz, Hakim Ferroukhi, Dimitri Rochman, Alexander Vasiliev

In this study, an optimization of the canister loading for used nuclear fuels is performed, solely based on their decay heat values. By taking into account the individual irradiation history for each fuel assembly, as well as with a number of assumptions o ...

ELSEVIER SCIENCE SA2020

Development and verification of pin-by-pin homogenized simplified transport solver Tortin for PWR core analysis

Andreas Pautz, Petra Mala

Currently, the pin-by-pin homogenized solvers are a very active research field as they can, unlike the nodal codes, directly predict the local power, while requiring significantly less computational resources than the heterogeneous transport codes. This pa ...

2020

Structural Snapshots of Cluster Growth from {U6 } to {U38 } During the Hydrolysis of UCl4

Marinella Mazzanti, Farzaneh Fadaei Tirani, Lucile Sylvie Danielle Chatelain, Radmila Faizova

Herein we report the assembly of large uranium(IV) clusters with novel nuclearities and/or shapes from the controlled hydrolysis of UCl4 in organic solution and in the presence of the benzoate ligands. {U6}, {U13}, {U16}, {U24}, {U38} oxo and oxo/hydroxo c ...

Wiley-VCH Verlag GmbH2019

Growth, Integration, and Functional Characterization of AlScN Thin Films for RF MEMS Devices

Mohammad Fazel Parsapour Kolour

Mobile communication has grown explosively in recent years, leading to a strong demand for cheap, but high-performing bandpass filters with low insertion loss and smaller size. Surface acoustic wave (SAW) and thin film bulk acoustic wave (BAW) resonators r ...

EPFL2019

Statistical Burnup Distribution Of Moving Pebbles In Htr-Pm Reactor

Andreas Pautz, Jiri Krepel, Fanny Vitullo, Horst-Michael Prasser

In the pebble-bed high temperature reactor under construction in China, called HTR-PM, the spherical fuel elements continuously flow downward in the cylindrical core. After the discharge, the burnup of each pebble is checked at the core outlet and, accordi ...

AMER SOC MECHANICAL ENGINEERS2018

Pin-by-Pin Treatment of LWR Cores with Cross Section Equivalence Procedures and Higher-Order Transport Methods

Petra Mala

This thesis presents a systematic study on the merits and limitations on using pin-by-pin resolution and transport theory based approaches for nuclear core design calculations. Starting from the lattice codes and an optimal cross section generation scheme, ...

EPFL2018

Modelling of fuel fragmentation, relocation and dispersal during Loss-of-Coolant Accident in Light Water Reactor

Vladimir Vladimirov Brankov

Recent LOCA tests with high burnup fuel at the OECD Halden Reactor Project and at Studsvik demonstrated the susceptibility of the fuel to fragment to small pieces, to relocate and possibly cause a hot-spot effect and to be dispersed in the event of claddin ...

EPFL2017

Analysis of reactivity worths of burnt PWR fuel samples measured in LWR-PROTEUS Phase II using a CASMO-5 reflected-assembly model

Mathieu Hursin, Hakim Ferroukhi, Daniel Jerôme Siefman

The reactivity loss of PWR fuel with burnup has been investigated experimentally by measuring the reactivity worths of highly-burnt fuel samples in a PWR test lattice in the framework of the LWR-PROTEUS Phase II program. Seven UO2 samples cut from fuel rod ...

2017

Metal-organic framework with optimally selective xenon adsorption and separation

Berend Smit, Cory Matthew Simon, Jian Liu

Nuclear energy is among the most viable alternatives to our current fossil fuel-based energy economy. The mass deployment of nuclear energy as a low-emissions source requires the reprocessing of used nuclear fuel to recover fissile materials and mitigate r ...

Nature Publishing Group2016

Isolation of a Star-Shaped Uranium(V/VI) Cluster from the Anaerobic Photochemical Reduction of Uranyl(VI)

Rosario Scopelliti, Marinella Mazzanti, Lucile Sylvie Danielle Chatelain

Actinide oxo clusters are an important class of compounds due to their impact on actinide migration in the environment. The photolytic reduction of uranyl(VI) has potential application in catalysis and spent nuclear fuel reprocessing, but the intermediate ...

Wiley-VCH Verlag GmbH2016

Products of in situ corrosion of depleted uranium ammunition in Bosnia and Herzegovina soils

Rizlan Bernier-Latmani, Barbora Bártová, Yuheng Wang, Konstantin von Gunten

Hundreds of tons of depleted uranium (DU) ammunition were used in previous armed conflicts in Iraq, Bosnia and Herzegovina, and Serbia/Kosovo. The majority (>90%) of DU penetrators miss their target and, if left in the environment, corrode in these postcon ...

Amer Chemical Soc2016

Mechanism of uranium reduction and immobilization in Desulfovibrio vulgaris biofilms

Rizlan Bernier-Latmani, Malgorzata Alicja Stylo

The prevalent formation of noncrystalline U(IV) species in the subsurface and their enhanced susceptibility to reoxidation and remobilization, as compared to crystalline uraninite, raise concerns about the long-term sustainability of the bioremediation of ...

Amer Chemical Soc2015

Trace concentration - Huge impact: Nitrate in the calcite/Eu(III) system

Kislon Voitchovsky, Moritz Schmidt

The interactions of trivalent lanthanides and actinides with secondary mineral phases such as calcite is of high importance for the safety assessment of deep geological repositories for high level nuclear waste (HLW). Due to similar ionic radii, calcium-be ...

Elsevier2014